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Record W1962114600 · doi:10.1007/s10874-015-9316-2

Chemical and isotopic interpretation of major ion compositions from precipitation: a one-year temporal monitoring study in Wrocław, SW Poland

2015· article· en· W1962114600 on OpenAlexaff
Monika Ciężka, Magdalena Modelska, Maciej Górka, Adriana Trojanowska, David Wîdory

Bibliographic record

VenueJournal of Atmospheric Chemistry · 2015
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicGroundwater and Isotope Geochemistry
Canadian institutionsUniversité du Québec à Montréal
FundersUniwersytet Wrocławski
KeywordsAmmoniumPrecipitationEnvironmental chemistryEquilibrium fractionationChemical compositionIsotopes of nitrogenNitrogenNitrateMineralization (soil science)Stable isotope ratioAerosolEnvironmental scienceFractionationChemistryAtmospheric sciencesIsotope fractionationGeologyMeteorology

Abstract

fetched live from OpenAlex

The chemical compositions (Na+, NH4 +, K+, Mg2+, Ca2+, Cl−, NO2 −, NO3 −, SO4 2−, HCO3 −) of wet precipitation and nitrogen isotope compositions δ15N(NH4 +) were studied from January to December 2010 in Wrocław (SW Poland). Results of a principle component analysis show that 82 % of the data variability can be explained by three main factors: 1) F1 (40 %) observed during vegetative season (electrical conductivity, HCO3 −, NO3 −, NO2 −, NH4 + and SO4 2−), mainly controlling rainwater mineralization; 2) F2 (26 %) observed during vegetative and heating seasons (K+, Ca2+ and Mg2+), probably representing a combination of two processes: anthropogenic dusts and fertilizers application in agricultural fields, and 3) F3 (16 %) reported mainly during heating season (Na+ and Cl−) probably indicating the influence of marine aerosols. Variations of δ15N(NH4 +) from −11.5 to 18.5 ‰ identify three main pathways for the formation of NH4 +: 1) equilibrium fractionation between NH3 and NH4 +; 2) kinetic exchange between NH3 and NH4 +; 3) NH4 + exchange between atmospheric salts particles and precipitation. The coupled chemical/statistical analysis and δ15N(NH4 +) approach shows that while fossil fuels burning is the main source of NH4 + in precipitation during the heating season, during the vegetative season NH4 + originates from local sewage irrigation fields in Osobowice or agricultural fertilizers.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.031
Threshold uncertainty score0.062

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.227
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations39
Published2015
Admission routes1
Has abstractyes

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