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Record W1972699526 · doi:10.1021/ac800149d

Multiple Surface Plasmon Resonances and Near-Infrared Field Enhancement of Gold Nanowells

2008· article· en· W1972699526 on OpenAlexaff
Kebin Li, Liviu Clime, Li‐Lin Tay, Bo Cui, Matthias Geißler, Teodor Veres

Bibliographic record

VenueAnalytical Chemistry · 2008
Typearticle
Languageen
FieldMaterials Science
TopicGold and Silver Nanoparticles Synthesis and Applications
Canadian institutionsNational Research Council CanadaInstitute for Microstructural Sciences
FundersGenomic Health
KeywordsRhodamine 6GDiscrete dipole approximationRaman scatteringPlasmonChemistrySurface plasmon resonanceExcitationNanosphere lithographyLocalized surface plasmonElectron-beam lithographySurface plasmonWavelengthOptoelectronicsOpticsDipoleMolecular physicsRaman spectroscopyNanotechnologyMaterials scienceNanoparticlePhysics

Abstract

fetched live from OpenAlex

Arrays of Au nanowells (NWs) were fabricated by electron-beam lithography (EBL) and characterized by surface plasmon resonance (SPR) and surface-enhanced Raman scattering (SERS). It is revealed that these Au NW arrays exhibit multiple SP resonances that can be tuned by adjusting the geometrical characteristics of the NWs. SERS activity of Au NWs was confirmed for a range of excitation wavelengths and a number of model compounds including rhodamine 6G (R6G), phthalazine, and single-stranded oligonucleotides. According to numerical simulations based on the discrete dipole approximation (DDA), SERS enhancement originates from high electromagnetic fields (hot spots) localized both inside and outside individual NWs. In addition, far-field intercoupling effects between NWs have been observed experimentally in arrays with subwavelength pitch sizes. We show that the SERS enhancement factors can also be tuned and optimized by adjusting the geometry of NWs.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.604

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.232
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations44
Published2008
Admission routes1
Has abstractyes

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