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Record W1981303914 · doi:10.1002/cjoc.200990174

Electrocatalytic Carboxylation of Benzyl Chloride at Silver Cathode in Ionic Liquid BMIMBF<sub>4</sub>

2009· article· en· W1981303914 on OpenAlexaff
Dongfang Niu, Jingbo Zhang, Kai Zhang, Teng Xue, Jiaxing Lu

Bibliographic record

VenueChinese Journal of Chemistry · 2009
Typearticle
Languageen
FieldChemical Engineering
TopicIonic liquids properties and applications
Canadian institutionsTellabs (Canada)
Fundersnot available
KeywordsChemistryIonic liquidTetrafluoroborateCyclic voltammetryCarboxylationPhenylacetic acidInorganic chemistryYield (engineering)ChlorideElectrochemistryCathodeBenzyl chlorideIonic bondingElectrodeOrganic chemistryIonCatalysisPhysical chemistryMetallurgy

Abstract

fetched live from OpenAlex

Abstract The feasibility of electrocarboxylation of benzyl chloride has been investigated at silver cathode in CO2‐saturated room‐temperature ionic liquid 1‐butyl‐3‐methylimidazolium tetrafluoroborate (BMIMBF4) solution for the first time. The electrochemical behavior was studied at different electrodes by cyclic voltammetry, which showed significant electrocatalytic effect of the silver electrode on the reduction of benzyl chloride. The highest yield of 45% of phenylacetic acid was obtained under optimal conditions. The recovered ionic liquid was reused for four times with gradual decrease in the yield of phenylacetic acid.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.218
Teacher spread0.213 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations37
Published2009
Admission routes1
Has abstractyes

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