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Record W1981303914 · doi:10.1002/cjoc.200990174

Electrocatalytic Carboxylation of Benzyl Chloride at Silver Cathode in Ionic Liquid BMIMBF<sub>4</sub>

2009· article· en· W1981303914 on OpenAlex
Dongfang Niu, Jingbo Zhang, Kai Zhang, Teng Xue, Jiaxing Lu

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueChinese Journal of Chemistry · 2009
Typearticle
Languageen
FieldChemical Engineering
TopicIonic liquids properties and applications
Canadian institutionsTellabs (Canada)
Fundersnot available
KeywordsChemistryIonic liquidTetrafluoroborateCyclic voltammetryCarboxylationPhenylacetic acidInorganic chemistryYield (engineering)ChlorideElectrochemistryCathodeBenzyl chlorideIonic bondingElectrodeOrganic chemistryIonCatalysisPhysical chemistryMetallurgy

Abstract

fetched live from OpenAlex

Abstract The feasibility of electrocarboxylation of benzyl chloride has been investigated at silver cathode in CO 2 ‐saturated room‐temperature ionic liquid 1‐butyl‐3‐methylimidazolium tetrafluoroborate (BMIMBF 4 ) solution for the first time. The electrochemical behavior was studied at different electrodes by cyclic voltammetry, which showed significant electrocatalytic effect of the silver electrode on the reduction of benzyl chloride. The highest yield of 45% of phenylacetic acid was obtained under optimal conditions. The recovered ionic liquid was reused for four times with gradual decrease in the yield of phenylacetic acid.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.605

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.218
Teacher spread0.213 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it