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Record W1987226223 · doi:10.1016/j.egypro.2014.11.312

Evolution of formation water chemistry and geochemical modelling of the CO2CRC Otway Site residual gas saturation test

2014· article· en· W1987226223 on OpenAlexaff
Dirk Kirste, Ralf R. Haese, Christopher J. Boreham, U. Schacht

Bibliographic record

VenueEnergy Procedia · 2014
Typearticle
Languageen
FieldEnvironmental Science
TopicCO2 Sequestration and Geologic Interactions
Canadian institutionsSimon Fraser University
FundersLawrence Berkeley National LaboratoryAustralian GovernmentAustralian National Low Emissions Coal Research and Development
KeywordsDissolutionSaturation (graph theory)CarbonateAlkalinityMineralogyChemical compositionGeochemical modelingChemistrySilicateCalciteGeology

Abstract

fetched live from OpenAlex

The CO 2 CRC Otway Project Stage 2B field test was a residual CO 2 saturation and dissolution experiment carried out on the Paaratte Formation in the Otway Basin of Australia. During the 87 day test a downhole U-tube sampling assembly was used to collect formation water samples at various time intervals. The waters were analysed for chemical composition, dissolved gas content and stable isotopic composition of H and O. Changes in the chemical and isotopic composition of the formation water were observed from the initial baseline samples collected through to the conclusion of the test. Systematic reoccurrences of relatively large linear changes in the alkalinity, Ca 2+ , Fe 2+ , Mg 2+ and SiO2(aq) were observed during different test sequences. Similar behaviour occurred for the δ 18 O and δ 2 H values suggesting a complex system controlled by at least two processes. The chemical evolution was consistent with CO 2 -water-rock interactions, dominated by carbonate dissolution with some silicate dissolution. The mineral dissolution driven changes in water composition are overlain by what was clearly mixing of the injected and in situ formation water. The isotopic composition of the water was used to confirm the role of mixing and the calculated residual gas saturation values were broadly consistent with those derived by other methods. The extent of reaction in the relatively short time frame of the test was used to evaluate the capabilities of kinetics based reaction path models. The models were generated using published reaction rate data with commonly used assumptions regarding upscaling of reactive surface area. These assumptions consist of reducing the calculated geometric surface area that accounts for grain shape and roughness by factors of 100 to 1000 depending on the mineral habit. The numerical models provided a very good fit to the field data indicating that the rate data and the associated assumptions are relatively robust.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.145
Threshold uncertainty score0.152

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.171
Teacher spread0.166 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2014
Admission routes1
Has abstractyes

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