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Record W1988489211 · doi:10.1021/ie010793d

A General Expression for the Ordered-Packed Volume Fraction of Hard Spheres of Different Diameters

2002· article· en· W1988489211 on OpenAlexaff
Cyrus Ghotbi, Juan H. Vera

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2002
Typearticle
Languageen
FieldEngineering
TopicPhase Equilibria and Thermodynamics
Canadian institutionsMcGill University
Fundersnot available
KeywordsMixing (physics)Hard spheresSPHERESVolume fractionComponent (thermodynamics)Atomic packing factorThermodynamicsFraction (chemistry)Binary numberLimit (mathematics)Value (mathematics)ChemistryVolume (thermodynamics)Statistical physicsPhysicsMathematicsMathematical analysisChromatographyStatisticsCrystallography

Abstract

fetched live from OpenAlex

An expression is proposed to evaluate the ordered-packed volume fraction of hard spheres of unequal diameters in multicomponent mixtures. This value can be used with different mixing rules and with any one-component hard-sphere equation of state (EOS) meeting the correct close-packed limit. It is shown that the new method improves the results produced by conventional mixing rules for the individual radial distribution functions (RDFs) at contact value of hard-sphere mixtures. Particular attention is given to the case of the large diameter ratio especially when the larger spheres are at low concentration. Based on the observation that, in a binary mixture, the value of the RDF at contact value of the larger spheres approaches the value of the RDF at contact value of a one-component hard-sphere fluid, the proposed expression is used to correct the RDF at contact value of a pure hard-sphere fluid in the Santos et al. mixing rule. The EOS obtained by combining the Ghotbi−Vera one-component EOS with the corrected Santos et al. mixing rule is used to predict different thermodynamic properties, and the results are compared with the computer-simulated data.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.002
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: none
Teacher disagreement score0.002
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.002
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0020.001
Science and technology studies0.0000.001
Scholarly communication0.0010.002
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0020.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.088
GPT teacher head0.291
Teacher spread0.203 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2002
Admission routes1
Has abstractyes

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