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Record W1991093672 · doi:10.2118/144097-ms

Shale Gas-in-Place Calculations Part II — Multi-component Gas Adsorption Effects

2011· article· en· W1991093672 on OpenAlexaff
R. C. Hartman, Ray J. Ambrose, I. Yücel Akkutlu, Christopher R. Clarkson

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldEngineering
TopicHydrocarbon exploration and reservoir analysis
Canadian institutionsUniversity of Calgary
Fundersnot available
KeywordsAdsorptionSorptionLangmuirVolume (thermodynamics)Real gasChemistryLangmuir adsorption modelComponent (thermodynamics)Shale gasOil shaleGas phaseNanoporousThermodynamicsChemical engineeringOrganic chemistryGeologyPhysics

Abstract

fetched live from OpenAlex

Abstract Recent studies have shown that shale gas industry is incorrectly determining gas-in-place volumes in reservoirs with a large sorption capacity by not properly accounting for the volume occupied by the adsorbed phase. Scanning electron microscopy has discovered nanopores in organic-rich shale with sizes typically in 3–100 nm range; adsorption data show presence of smaller pores and micropores (< 2 nm) as part of the predicted pore size distributions. At pore diameters of this scale the adsorption potential is high and thus the fractional pore volume occupied by adsorbed gas is often substantial. Hence a portion of the total pore volume would be occupied by the adsorbed gas and not available for the free gas molecules. In SPE 131772 a volumetric method, which accounts for the pore volumes occupied by the adsorbed and free gases, has been proposed based on single-component Langmuir adsorption model. In SPE 141416 we recognized the importance and impact of multi-component gas adsorption potential and adsorbed gas density when calculating gas-in-place estimates. We combined the widely used yet thermodynamically inconsistent Extended Langmuir model with volumetrics and free gas composition to formulate a new gas-in-place equation that accounts for the pore space taken up by a multi-component adsorbed gas phase. This paper extends the discussions on the adsorption layer effect of multi-component natural gases. The approach is based on thermodynamically-consistent ideal adsorbed solution (IAS) model to accurately predict adsorbed gas storage capacity for gas mixtures. We expanded on our previous work, where we calculated single-component adsorbed-phase density using molecular modeling and Monte Carlo simulation methods, and propose a new equation-of-state-based analytical approach to predict the adsorbed-phase density of a mixture. In concert, the model improves accuracy of the gas-in-place equations needed to account for the pore space taken up by a multi-component adsorbed phase. The new method yields total gas-in-place predictions, which suggest that an adjustment is necessary in volume calculations, especially for gas shales with high C2+ composition and high in total organic content. The new method is therefore recommended for shale gas-in-place calculations.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.103
Threshold uncertainty score0.599

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.025
GPT teacher head0.223
Teacher spread0.198 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations80
Published2011
Admission routes1
Has abstractyes

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