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Record W1992442226 · doi:10.1021/jp066800z

Exclusion of Salt Solutions from Activated Carbon Pores and the Relationship to Contact Angle on Graphite

2007· article· en· W1992442226 on OpenAlexaff
Philippe Westreich, H. Fortier, Stephanie Flynn, Stephen Foster, J. R. Dahn

Bibliographic record

VenueThe Journal of Physical Chemistry C · 2007
Typearticle
Languageen
FieldMaterials Science
TopicGraphene research and applications
Canadian institutionsDalhousie University
Fundersnot available
KeywordsGraphiteContact angleSalt (chemistry)Carbon fibersAdsorptionActivated carbonChemical engineeringSalt solutionIncipient wetness impregnationMaterials scienceChemistryInorganic chemistryComposite materialOrganic chemistryCatalysisComposite number

Abstract

fetched live from OpenAlex

The exclusion of salts from the pores of activated carbon granules is demonstrated for the first time for the salts K 2 CO 3, K 2 HPO 4 and K 3 PO 4 . In soaking experiments, the concentrations of solutions of K 2 CO 3, K 2 HPO 4, and K 3 PO 4 inside the pores are less than in the bulk solutions. This phenomenon is observed by measuring the bulk concentration, which increases upon addition of carbon. This suggests that these salts are repelled by the carbon surface. In incipient wetness experiments, the three aforementioned salts do not enter the carbon at concentrations greater than ∼1 M. The contact angles of these three salt solutions on highly oriented pyrolitic graphite and polished resin-impregnated graphite surfaces rise with concentration and approach 90°, which suggests that these solutions would not enter activated carbon pores. By contrast, soaking, incipient wetness, and contact angle measurements for salts like ZnCl 2 and Zn(CH 3 COO) 2 show preferential adsorption by soaking (the salt is depleted from the solution), high imbibing limits (maximum incipient wetness volumes) at high solution concentrations, and a reduction of contact angle with increase in concentration. It is found that the behavior of these solutions on graphite surfaces approximates the solution behavior on an activated carbon that is relatively low in acidic surface functional groups.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0010.000
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.289
Teacher spread0.266 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations26
Published2007
Admission routes1
Has abstractyes

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Same venueThe Journal of Physical Chemistry CSame topicGraphene research and applicationsFrench-language works237,207