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Record W1993199492 · doi:10.1021/ma001080u

Morphology of Poly(2-ethylhexyl methacrylate):Poly(butyl methacrylate) Latex Blend Films

2001· article· en· W1993199492 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueMacromolecules · 2001
Typearticle
Languageen
FieldEngineering
TopicMaterial Properties and Processing
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsMethacrylateMorphology (biology)Materials sciencePulmonary surfactantDispersion (optics)Chemical engineeringCopolymerPolymer chemistryPolymerPhase (matter)Composite materialChemistryOrganic chemistryOptics

Abstract

fetched live from OpenAlex

This paper describes the morphology of the latex films formed from a mixture of two different latex particles: poly(butyl methacrylate) (PBMA, 120 nm) and poly(2-ethylhexyl methacrylate) (PEHMA, 100 nm). Twenty percent of the PBMA phase is labeled with 1 mol % anthracene. Using confocal fluorescence microscopy, we obtained images of the internal morphology of the dry films. Atomic force microscopy was used to image the surfaces of the films. For the same blend composition, 10 wt % PBMA and 90 wt % PEHMA, we studied the effect of two factors on the blend morphology: the presence or the absence of the surfactant SDS (ca. 2 wt % of the weight of polymers) in the dispersion and the dispersion concentration. We related the different morphologies we observed to the differences in the drying mechanisms. In the case of a surfactant-free film cast from a 5 wt % dispersion mixture, the film dried homogeneously, and we observed uniform distribution of the PBMA dispersed phase in the PEHMA matrix. In the presence of surfactant, the film dries laterally with a propagating drying front, and we observed network-like structures formed by PBMA particles in a matrix of PEHMA. The segregation of PBMA and PEHMA particles can be explained by differences in the surfactant adsorption onto PBMA and PEHMA particles.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.034
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.226
Teacher spread0.213 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it