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Record W1994133850 · doi:10.1021/ie010135t

Hydrogen Production by Steam Reforming of Vegetable Oils Using Nickel-Based Catalysts

2001· article· en· W1994133850 on OpenAlexfundno aff
Maximiliano Marquevich, Xavier Farriol, F. Medina, Daniel Montané

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2001
Typearticle
Languageen
FieldEngineering
TopicCatalysis and Hydrodesulfurization Studies
Canadian institutionsnot available
FundersNational Renewable Energy LaboratoryUniversité de Sherbrooke
KeywordsSteam reformingCatalysisVegetable oilHydrogenHydrogen productionChemistrySoybean oilBiomass (ecology)Methane reformerChemical engineeringPulp and paper industryMaterials scienceOrganic chemistryFood scienceAgronomy

Abstract

fetched live from OpenAlex

Vegetable oils and fats are a renewable resource derived from biomass that can contribute to reduce the net emission of CO 2 into the atmosphere if used to produce hydrogen for fuel-cell-based energy systems. In this paper, we present the results of the steam reforming of several vegetable oils with three different nickel-based commercial catalysts (ICI 46-1, ICI 46-4, and UCI G90C) and two research catalysts (UdeS and HT). The experiments were performed in an isothermal fixed-bed tubular reactor at steam-to-carbon ( S / C ) ratios of 9, 6, and 3 and temperatures between 500 and 630 °C. High space velocities of 0.76−1.90 mol carbon /(g cat h) were used so that conversions of the feed would be incomplete. Hydrogen productions were from 0.3 to 7.5 mol H 2 /(g Ni h) depending on the operating conditions. The HT catalyst, which was prepared from a hydrotalcite-like precursor, seems promising for steam reforming vegetable oils because of its very high activity per gram of catalyst. Results for the steam reforming of sunflower, rapeseed, corn, and soybean oils at the same catalyst temperature and S / C ratio show that oil conversion to gases and hydrogen yields do not depend on the type of vegetable oil. This indicates that the process might be suitable for producing hydrogen from residual oils and fats from food processing, for which process economics are more favorable.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.184
Threshold uncertainty score0.966

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.084
GPT teacher head0.308
Teacher spread0.223 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations38
Published2001
Admission routes1
Has abstractyes

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