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Record W2002428671 · doi:10.1021/cm010171i

Incorporation of Cyclodextrin into Mesostructured Silica

2001· article· en· W2002428671 on OpenAlexaff
Ragibul Huq, Louis Mercier, Patricia J. Kooyman

Bibliographic record

VenueChemistry of Materials · 2001
Typearticle
Languageen
FieldMaterials Science
TopicMesoporous Materials and Catalysis
Canadian institutionsLaurentian University
Fundersnot available
KeywordsMesoporous materialMesoporous silicaCyclodextrinAqueous solutionMesoporous organosilicaChemical engineeringTransmission electron microscopyAdsorptionMaterials scienceGraftingChemistryPulmonary surfactantInorganic chemistryNuclear chemistryNanotechnologyOrganic chemistryCatalysis

Abstract

fetched live from OpenAlex

The incorporation of cyclodextrin (CD) groups inside mesoporous silica frameworks was attempted using two methods: by the grafting of the CD groups into the channels of preformed mesoporous silica hosts and by the direct synthesis of CD-containing mesoporous materials by a one-step process. While the grafting procedure failed to incorporate CD groups inside the pore channels of mesoporous silica substrates, the direct synthesis approach yielded materials whose physical and chemical characteristics (as determined by X-ray diffraction, N 2 sorptometry, transmission electron microscopy, and elemental analysis) were indicative of the presence of CD groups inside the pore channels of the materials. The CD-containing mesoporous materials, denoted as CD-HMS, were prepared by the co-condensation of tetraethoxysilane and a silylated derivative of β-cyclodextrin in the presence of a structure-directing dodecylamine surfactant solution. Materials with CD group loadings up to 0.39 mmol g -1 and uniform pore channels with diameters in the range of 38−42 Å were prepared by this method. Preliminary adsorption experiments using aqueous p -nitrophenol solutions showed that the CD-HMS materials were promising for the removal of organic compounds from water.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.008
Threshold uncertainty score0.993

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0080.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.227
Teacher spread0.219 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations104
Published2001
Admission routes1
Has abstractyes

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