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Record W2005049876 · doi:10.1021/je8008073

Comparison between Experimental and Theoretical Estimations of the Thermal Expansion, Concentration Expansion Coefficients, and Viscosity for Binary Mixtures under Pressures up to 20 MPa

2009· article· en· W2005049876 on OpenAlexaff
Henri Bataller, Christelle Miqueu, Frédéric Plantier, Jean‐Luc Daridon, T. J. Jaber, Alireza Abbasi, M. Ziad Saghir, M. Mounir Bou‐Ali

Bibliographic record

VenueJournal of Chemical & Engineering Data · 2009
Typearticle
Languageen
FieldEngineering
TopicPhase Equilibria and Thermodynamics
Canadian institutionsToronto Metropolitan University
Fundersnot available
KeywordsThermal expansionChemistryThermodynamicsBinary numberViscosityWork (physics)Equation of stateVolume (thermodynamics)PhysicsMathematics

Abstract

fetched live from OpenAlex

In this work, we have measured the densities of binary mixtures of n -dodecane, 1-phenyl-2-methylpropane, and 1,2,3,4-tetrahydronaphthalene for pressures varying from (0.1 to 20) MPa at an average temperature of 25 °C. By a derivative method, we have determined the thermal expansion and concentration expansion coefficients for binary mixtures of equal mass fraction. In addition, viscosities have been measured and compared with theoretical estimates. To accurately predict the thermal expansion and concentration expansion coefficients, the densities of the binary mixtures were calculated using PC-SAFT, Peng-Robinson, and volume translated Peng-Robinson equations of state. The comparison with measured densities showed that PC-SAFT has a better agreement with experimental data than the other equations of state. From calculated densities we evaluated the thermal expansion and concentration expansion variation coefficients. We have found that PC-SAFT gives a suitable prediction for the two derivative properties unlike the two other equations of state. The combination of the model of Lohrenz-Bray-Clark for the viscosity of liquid mixtures and the densities calculated with the three equations of state gave a poor prediction of the viscosities of the binary mixtures.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.471
Threshold uncertainty score0.356

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.295
Teacher spread0.276 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations15
Published2009
Admission routes1
Has abstractyes

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