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Record W2006774265 · doi:10.1021/ie020738k

Determination of the Structural Features of Distinct Amines Important for the Absorption of CO<sub>2</sub> and Regeneration in Aqueous Solution

2003· article· en· W2006774265 on OpenAlexafffund
Danielle Bonenfant, Murielle Mimeault, Robert Hausler

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2003
Typearticle
Languageen
FieldEngineering
TopicCarbon Dioxide Capture Technologies
Canadian institutionsUniversité du Québec à Montréal
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsAlkanolamineTriethanolaminePyrrolidineChemistryDesorptionAqueous solutionAbsorption (acoustics)Amine gas treatingPyridineTriethylamineAdsorptionCarbon dioxideTertiary amineOrganic chemistryMaterials scienceAnalytical Chemistry (journal)

Abstract

fetched live from OpenAlex

A study of carbon dioxide (CO 2 ) absorption/desorption has been carried out to estimate the influence of the structural features of distinct amines on their CO 2 absorption and regeneration. The absorption has been made at two different CO 2 flow rates with a series of aqueous 5 wt % ammonia, monoethanolamine (MEA), triethanolamine (TEA), triethylamine, pyridine, pyrrolidine, 2-(2-aminoethylamino)ethanol (AEE), and N -(2-aminoethyl)-1,3-propanediamine (AEPDNH 2 ) solutions, while the CO 2 desorption has been performed by heating these solutions. The presence of two or three amino groups in AEE and AEPDNH 2, the structure of tertiary amine and alkanolamine, and a nonaromatic ring of pyrrolidine might favor the CO 2 absorption, while the structural features of ammonia and pyridine seem to be unfavorable. The tertiary alkanolamine is the most easy to regenerate and looses less of its CO 2 loading after regeneration. It appears that AEE and AEPDNH 2 would represent interesting compounds which could be used as CO 2 absorbents in industrial technologies to prevent CO 2 release into the atmosphere.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.034
GPT teacher head0.278
Teacher spread0.244 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations189
Published2003
Admission routes2
Has abstractyes

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