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Record W2007365510 · doi:10.1002/macp.200300121

Butyl Acrylate/Vinyl Acetate Miniemulsion Polymerization: A Study on Compartmentalization

2004· article· en· W2007365510 on OpenAlexafffund
Renata Jovanović, Marc A. Dubé

Bibliographic record

VenueMacromolecular Chemistry and Physics · 2004
Typearticle
Languageen
FieldChemistry
TopicAdvanced Polymer Synthesis and Characterization
Canadian institutionsUniversity of Ottawa
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsMiniemulsionMonomerVinyl acetatePolymerizationPolymer chemistryButyl acrylateAcrylateCopolymerEmulsion polymerizationChemistryPolymerRadical polymerizationMaterials scienceChemical engineeringOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Summary: A series of butyl acrylate/vinyl acetate miniemulsions were investigated. Two procedures were used to prepare the miniemulsions: one in which the monomers were mixed together, sonicated, and polymerized, and the other, in which the individual monomers were sonicated prior to mixing and then polymerized. Kinetic and final properties of the obtained polymers were compared. The two procedures offer interesting insights into monomer compartmentalization in miniemulsions. In most cases, there were no differences in monomer conversion, copolymer composition, particle size or average molecular weights between the two procedures. ATR‐FTIR spectroscopy was used to assess possible monomer transfer. The spectra obtained from each polymerization procedure were compared and no evidence of compartmentalization was found. Both procedures yielded similar spectra indicating that monomer transfer between particles occurred. In addition, adhesive properties of the obtained latexes were investigated. Due to the fact that relatively large amounts of CTA were used, adhesive performance was poor. Comparison of the spectra of miniemulsion polymerizations obtained by two different procedures (BA/VAc 85/15 wt/wt). image Comparison of the spectra of miniemulsion polymerizations obtained by two different procedures (BA/VAc 85/15 wt/wt).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.011
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.239
Teacher spread0.229 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2004
Admission routes2
Has abstractyes

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