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Record W2009990712 · doi:10.1021/ie040253r

Comparative Analysis of the Carbon Dioxide Absorption and Recuperation Capacities in Aqueous 2-(2-Aminoethylamino)ethanol (AEE) and Blends of Aqueous AEE and <i>N</i>-Methyldiethanolamine Solutions

2005· article· en· W2009990712 on OpenAlexfundno aff
Danielle Bonenfant, Murielle Mimeault, Robert Hausler

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2005
Typearticle
Languageen
FieldEngineering
TopicCarbon Dioxide Capture Technologies
Canadian institutionsnot available
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsDesorptionAqueous solutionChemistryCarbon dioxideAbsorption (acoustics)Amine gas treatingEthanolAnalytical Chemistry (journal)ChromatographyNuclear chemistryOrganic chemistryAdsorptionMaterials science

Abstract

fetched live from OpenAlex

A study of carbon dioxide (CO 2 ) absorption/desorption has been carried out in diverse aqueous amine solutions consisting of 2-(2-aminoethylamino)ethanol (AEE), monoethanolamine (MEA), and the blends of AEE and N -methyldiethanolamine (MDEA) at different concentrations to compare the CO 2 loading and recuperation properties of these amines. The CO 2 absorption loading has been estimated in 0.476, 0.951, 1.427, and 2.378 M AEE solutions, a 2.378 M MEA solution, and two blends of 1.427 M AEE + 0.418 M MDEA and 1.427 M AEE + 0.836 M MDEA with two CO 2 concentrations of 5.01 and 100 vol % at 23 °C and a flow rate of 3.067 L/min. The CO 2 desorption was performed by heating these solutions at 100−102 °C. The results revealed that the AEE diamine possesses a greater CO 2 absorption capacity than MEA while its CO 2 desorption capacity was inferior to that observed for MEA. Moreover, the CO 2 recuperation capacity obtained for AEE was greater than that of MEA at the same concentration. Interestingly, the CO 2 absorption in an aqueous AEE solution was also slightly increased in the presence of MDEA while its desorption was highly enhanced, resulting in an increase of about 15% of its CO 2 recuperation capacity. Taken together, these results suggest that the structural properties of AEE, including the presence of two amino groups, as compared to MEA could favor its CO 2 absorption and recuperation capacities. Therefore, AEE and the blends of AEE + MDEA could represent interesting absorbents for the development of new methods to eliminate the CO 2 emanation into the atmosphere by industrial combustion processing.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.038
Threshold uncertainty score0.917

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.055
GPT teacher head0.279
Teacher spread0.224 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations39
Published2005
Admission routes1
Has abstractyes

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