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Record W2011506992 · doi:10.1002/app.23046

Differential scanning calorimetry of copolymer of isotactic polypropylene backbone with grafted poly(ethylene‐<i>co</i>‐propylene) branches

2006· article· en· W2011506992 on OpenAlexaff
Philip M. Whitney, Shiping Zhu

Bibliographic record

VenueJournal of Applied Polymer Science · 2006
Typearticle
Languageen
FieldMaterials Science
TopicPolymer crystallization and properties
Canadian institutionsMcMaster University
Fundersnot available
KeywordsDifferential scanning calorimetryTacticityMaterials sciencePolymer chemistryEnthalpy of fusionPolypropyleneMelting pointCopolymerCrystallizationEnthalpyElectron paramagnetic resonanceEthylene propylene rubberEthylenePolymerAnalytical Chemistry (journal)ChemistryPolymerizationComposite materialThermodynamicsChromatographyOrganic chemistryNuclear magnetic resonance

Abstract

fetched live from OpenAlex

Abstract A series of graft polymers having polypropylene (PP) backbone and poly(ethylene‐co‐propylene) (EPR) side chains was prepared. PP backbone molecular weight (Mn) was 28–98 kg/mol, EPR side chain Mn was 2.6–17 kg/mol, and EPR content was 0–16 wt %. In this work, thermal analysis of the copolymers was performed using differential scanning calorimetry (DSC). Nonisothermal crystallization was performed at different cooling rates. The DSC thermograms revealed multiple melting peaks for slowly cooled samples, most likely the result of the melting of thinner tangential lamellae followed by the melting of thicker radial lamellae. Equilibrium melting temperature (Tm0) was determined using the linear Hoffman–Weeks method. Another approach was also used for determining Tm0: melting temperature (Tm) and crystallization temperature (Tc) were plotted as functions of logarithmic cooling rate. Linear relationships were observed for all samples with the cross points as Tm0's. As cooling rate decreased, Tc, Tm, and enthalpy of fusion (ΔHf) increased. Tm and Tm0 increased with increasing PP Mn. Tc and Tm were unaffected by the grafting of EPR onto the PP backbone. Tm0 and ΔHf decreased as EPR content increased. © 2006 Wiley Periodicals, Inc. J Appl Polym Sci 99: 3380–3388, 2006

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.221
Teacher spread0.214 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2006
Admission routes1
Has abstractyes

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