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Record W2014190157 · doi:10.1103/physrevb.64.075420

Conductance,<mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mi>I</mml:mi><mml:mo>−</mml:mo><mml:mi>V</mml:mi></mml:math>curves, and negative differential resistance of carbon atomic wires

2001· article· lv· W2014190157 on OpenAlexafffund
Brian Larade, Jeremy Taylor, H. Mehrez, Hong Guo

Bibliographic record

VenuePhysical review. B, Condensed matter · 2001
Typearticle
Languagelv
FieldEngineering
TopicMolecular Junctions and Nanostructures
Canadian institutionsMcGill University
FundersNatural Sciences and Engineering Research Council of CanadaMcGill University
KeywordsConductanceHOMO/LUMOElectrodeMaterials scienceThermal conductionAtomic physicsPhysicsAnalytical Chemistry (journal)Condensed matter physicsMoleculeChemistryThermodynamicsQuantum mechanics

Abstract

fetched live from OpenAlex

We report on a first-principles analysis of transport properties of carbon atomic wires in contact with two metallic electrodes under external bias. The equilibrium conductance of the atomic wires is found to be sensitive to two factors: charge transfer doping, which aligns the Fermi level of the electrodes to the lowest unoccupied molecular orbital (LUMO) of the carbon chain, and the overlapping of scattering states to the LUMO. The conductance is also affected by the crystalline orientation of the electrodes. The low-bias current-voltage $(I\ensuremath{-}V)$ characteristic is linear, but a negative differential resistance is observed at higher bias due to a shift of conduction channels relative to the states of the electrodes by the external bias potential. Our first-principles results give a clear physical picture of the molecule-electrode coupling, which is the controlling factor of electric conduction through the carbon atomic wires.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score0.016

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0050.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.240
Teacher spread0.229 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations204
Published2001
Admission routes2
Has abstractyes

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