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Record W2015312861 · doi:10.1063/1.4830401

Effect of an external electric field on the diffusion-influenced geminate reversible reaction of a neutral particle and a charged particle in three dimensions. III. Ground-state ABCD reaction

2013· article· en· W2015312861 on OpenAlexaff
Shang Yik Reigh

Bibliographic record

VenueThe Journal of Chemical Physics · 2013
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicDiffusion and Search Dynamics
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsChemistryElectric fieldLaplace transformDiffusionGround stateKinetic energyPower lawDomain (mathematical analysis)Field (mathematics)Particle (ecology)PhysicsAtomic physicsThermodynamicsQuantum mechanicsMathematical analysisMathematicsStatistics

Abstract

fetched live from OpenAlex

In the presence of an external electric field, the ground-state \documentclass[12pt]{minimal}\begin{document}$A+B^q \rightleftharpoons C^q + D$\end{document}A+Bq⇌Cq+D diffusion-influenced reversible reaction for a geminate pair, a neutral and a charged particle, is investigated in three dimensions. The probability density functions, the rates of reactions, and the survival probabilities of individual particles are analytically derived in the Laplace domain in terms of series solutions. The long-time kinetics of probability density functions and rates of reactions in rescaled forms shows a kinetic transition behavior from a t−3/2 power law to a t−3/2et increase when the condition \documentclass[12pt]{minimal}\begin{document}$D_1F_1^2 \le D_2F_2^2$\end{document}D1F12≤D2F22, which depends on the diffusivities of particles and the external electric fields, changes to \documentclass[12pt]{minimal}\begin{document}$D_1F_1^2 > D_2F_2^2$\end{document}D1F12>D2F22. In the transition region \documentclass[12pt]{minimal}\begin{document}$D_1F_1^2 = D_2F_2^2$\end{document}D1F12=D2F22, the long-time behavior also shows a t−3/2 power law decay but with a different value of the prefactor. The rescaled survival probabilities only exhibit an exponentially increasing behavior at long times with no dependence on the various values of parameters.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Theoretical or conceptual · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.014

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0040.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.246
Teacher spread0.239 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designTheoretical or conceptual
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations4
Published2013
Admission routes1
Has abstractyes

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