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Record W2021717779 · doi:10.1002/poc.1795

CO<sub>2</sub> production in the bromate‐1,4‐cyclohexanedione oscillatory reaction

2010· article· en· W2021717779 on OpenAlexafffund
Jiamin Feng, James R. Green, Samuel A. Johnson, Jichang Wang

Bibliographic record

VenueJournal of Physical Organic Chemistry · 2010
Typearticle
Languageen
FieldChemistry
TopicOxidative Organic Chemistry Reactions
Canadian institutionsUniversity of Windsor
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsChemistryBromateRing (chemistry)Gravimetric analysisSpectroscopyCarbon dioxidePhotochemistryMedicinal chemistryOrganic chemistryIon

Abstract

fetched live from OpenAlex

Abstract NMR and GC/MS spectroscopy of the organic extracts of the oscillatory bromate‐1,4‐cyclohexanedione reaction illustrate the presence of ring‐opening products 5‐(dibromomethylene)‐2(5H)‐furanone, (E)‐5,5,5‐tribromo‐4‐oxo‐2‐pentenoic acid, and dibromoacetic acid, particularly at elevated temperatures. The loss of a carbon atom from the six‐membered ring after ring opening led to gas formation and such a process became more vigorous at &gt;60 °C, with the direct observation of bubbles in a stirred batch reactor. Gravimetric experiments confirm that the amount of carbon dioxide gas produced increases rapidly with reaction temperature. Parallel experiments suggest that the ring‐opening process involves the oxidation of brominated benzoquinones by bromate. Copyright © 2010 John Wiley &amp; Sons, Ltd.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.002
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.233
Teacher spread0.226 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations7
Published2010
Admission routes2
Has abstractyes

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