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Record W2029154351 · doi:10.1021/la990710m

Characterization of Oil Droplets under a Polymer Film by Laser Scanning Confocal Fluorescence Microscopy

2000· article· en· W2029154351 on OpenAlexaff
José Paulo S. Farinha, Mitchell A. Winnik, Kenneth G. Hahn

Bibliographic record

VenueLangmuir · 2000
Typearticle
Languageen
FieldMaterials Science
TopicSurface Modification and Superhydrophobicity
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsMaterials scienceOil dropletContact angleTrioleinWettingPolymerChemical engineeringSubstrate (aquarium)Scanning electron microscopeDewettingAnalytical Chemistry (journal)Composite materialPolymer chemistryChemistryEmulsionChromatographyOrganic chemistry

Abstract

fetched live from OpenAlex

We studied the wetting behavior of thin oil films on quartz and poly(ethylene terephthalate) (PET) substrates before and after being coated with a polymer colloidal dispersion. The triolein oil was doped with a trace of a fluorescent dye, and the films were prepared by casting a dilute solution of dyed triolein in acetone onto the substrates. The films were then observed by laser scanning confocal fluorescence microscopy (LSCFM). On quartz, triolein breaks up into approximately spherical, micrometer-sized droplets as the acetone evaporates. The oil droplets were coated with a water dispersion of a film-forming latex dispersion of poly(butyl methacrylate) (PBMA). Most of the droplets adhered to the quartz substrate as the water evaporates. With LSCFM, we could image the triolein droplets under the transparent polymer latex film. These had larger volumes than those formed in air, and their micro-contact angle increased from 〈θ〉 = (32 ± 5)° at the quartz−air interface to 〈θ〉 = (71 ± 4)° at the quartz−PBMA interface. When deposited on PET, the triolein wets the substrate surface and forms an almost homogeneous film. Upon coating with a PBMA latex film, we observed some dewetting of the oil from the PET substrate, and the micro-contact angle of the oil increased from 〈θ〉 = (8 ± 4)° at the PET−air interface to 〈θ〉 = (18 ± 5)° at the PET−PBMA interface.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.008
Threshold uncertainty score0.995

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0060.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.237
Teacher spread0.226 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations17
Published2000
Admission routes1
Has abstractyes

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