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Record W2033045709 · doi:10.1149/1.1939211

Combinatorial Electrodeposition of Ternary Cu–Sn–Zn Alloys

2005· article· en· W2033045709 on OpenAlexaff
S. D. Beattie, J. R. Dahn

Bibliographic record

VenueJournal of The Electrochemical Society · 2005
Typearticle
Languageen
FieldEngineering
TopicElectrodeposition and Electroless Coatings
Canadian institutionsDalhousie University
Fundersnot available
KeywordsTernary operationMaterials scienceAlloyDeposition (geology)CopperElectrochemistryChemical engineeringElectrodeMetallurgyComputer scienceChemistryPhysical chemistry

Abstract

fetched live from OpenAlex

Active-inactive alloy systems (such as Cu–Sn–Zn) have been proposed to replace graphitic negative electrodes in commercial lithium-ion batteries due to their high theoretical capacity and relatively good cyclability. The performance of these electrode materials is largely determined by their composition. Identifying the optimal composition that provides both large capacity and good cyclability requires the testing of tens, hundreds or even thousands of different alloys. Combinatorial deposition and screening techniques lend themselves well to this kind of optimization study. Galvanostatic deposition in an electrochemical Hull cell is used to fabricate a composition-spread film of binary Sn–Zn alloys. A second step involving a water gun and weak copper sulfate solution is used to achieve a composition spread film of ternary Cu–Sn–Zn alloys. Energy-dispersive spectroscopy and X-ray diffraction are used to characterize the electrodeposited films. The significance and uniqueness of this work is illustrated by our ability to perform combinatorial material science simply and inexpensively. In addition, a phenomenological model is presented to describe the deposition process. The success of the phenomenological model demonstrates we have an understanding, albeit rudimentary, of the immersion deposition process.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.022
Threshold uncertainty score0.612

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.001
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.193
Teacher spread0.190 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations41
Published2005
Admission routes1
Has abstractyes

Explore more

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