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Record W2039493126 · doi:10.1021/ie504030v

Model for Surface Diffusion of Adsorbed Gas in Nanopores of Shale Gas Reservoirs

2015· article· en· W2039493126 on OpenAlexafffund
Keliu Wu, Xiangfang Li, Chenchen Wang, Wei Yu, Zhangxin Chen

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2015
Typearticle
Languageen
FieldEngineering
TopicHydrocarbon exploration and reservoir analysis
Canadian institutionsUniversity of Calgary
FundersMinistry of Science and Technology of the People's Republic of ChinaNatural Sciences and Engineering Research Council of CanadaNational Natural Science Foundation of ChinaAlberta Innovates - Technology FuturesCMG Reservoir Simulation Foundation
KeywordsKnudsen diffusionDiffusionAdsorptionDesorptionSurface diffusionChemistryMass transferNanoporeGaseous diffusionMacroporeSorptionKnudsen numberOil shaleMesoporous materialChemical engineeringThermodynamicsMaterials sciencePorosityChromatographyNanotechnologyGeologyPhysical chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

Surface diffusion plays a key role in gas mass transfer due to the majority of adsorbed gas within abundant nanopores of organic matter in shale gas reservoirs. Surface diffusion simulation is very complex as a result of high reservoir pressure, surface heterogeneity, and nonisothermal desorption in shale gas reservoirs. In this paper, a new model of surface diffusion for adsorbed gas in shale gas reservoirs is established, which is based on a Hwang model derived under a low pressure condition and considers the effect of adsorbed gas coverage under high pressure. Additionally, this new model considers the effects of surface heterogeneity, isosteric sorption heat, and nonisothermal gas desorption. Results show that (1) the surface diffusion coefficient increases with pressure and temperature, while it decreases with activation energy and gas molecular weight; (2) contributions of viscous flow, Knudsen diffusion, and surface diffusion to the total gas mass transfer are varying during the development of shale gas reservoirs, which are mainly controlled by nanopore-scale and pressure; (3) in micropores (pore radius of <2 nm), the contribution of surface diffusion to the gas mass transfer is dominant, up to 92.95%; in macropores (pore radius of >50 nm), the contribution is less than 4.39%, which is negligible; in mesopores (2 nm < pore radius < 50 nm), the contribution is between micropores and macropores.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.011
Threshold uncertainty score0.021

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.000
Science and technology studies0.0000.001
Scholarly communication0.0010.002
Open science0.0010.001
Research integrity0.0020.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.155
GPT teacher head0.327
Teacher spread0.172 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations344
Published2015
Admission routes2
Has abstractyes

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