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Record W2040035668 · doi:10.1021/jp012854r

Propagation Failure in an Array of Oregonator Cells and Irreversible Thermodynamics of an Assembly of Discrete Systems

2002· article· en· W2040035668 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueThe Journal of Physical Chemistry A · 2002
Typearticle
Languageen
FieldComputer Science
TopicNonlinear Dynamics and Pattern Formation
Canadian institutionsMcGill University
Fundersnot available
KeywordsWave propagationAmplitudePhysicsHomogeneousFront (military)Perturbation (astronomy)MechanicsThermodynamicsMeteorology

Abstract

fetched live from OpenAlex

In this paper we report on a numerical study of wave propagation and its failure in a one-dimensional array of coupled chemical cells and irreversible thermodynamics of the array. The Oregonator model for the Belousov−Zhabotinsky reaction is used to model the chemical reactions. In particular, we investigate the dependence of wave front propagation failure on the mass exchange rate for the Ce 4+ component between cells and on the amplitude of a perturbation employed to trigger a propagation of transition from an initially homogeneous state to final stationary patterns reached by the system. In the case of the Oregonator, there appear two critical mass transfer rates at which propagation failure occurs, in contrast to the cases of the cubic model or the sine-Gordon model reported in the literature. By following the evolution of the calortropy production accompanying wave propagation, we construct phase diagrams that provide valuable insights into the propagation failure phenomenon. The global calortropy production is shown to exhibit discontinuous changes with respect to the transfer rate when propagation failure occurs. When a complete propagation failure occurs, the global calortropy flux through the array vanishes, whereas it is nonvanishing when there is a partial or complete propagation of the wave front. When the calortropy flux vanishes, the wave front speed and the net mass flux between the cells also vanish.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.712
Threshold uncertainty score0.167

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.220
Teacher spread0.211 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it