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Record W2040059706 · doi:10.1039/b900300b

Structural and optical investigation of colloidal Ln3+/Yb3+ co-doped KY3F10 nanocrystals

2009· article· en· W2040059706 on OpenAlexafffund
Venkataramanan Mahalingam, Fiorenzo Vetrone, Rafik Naccache, Adolfo Speghini, John A. Capobianco

Bibliographic record

VenueJournal of Materials Chemistry · 2009
Typearticle
Languageen
FieldMaterials Science
TopicLuminescence Properties of Advanced Materials
Canadian institutionsConcordia University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsPhoton upconversionMaterials scienceNanocrystalRietveld refinementLanthanideDopingTransmission electron microscopyAnalytical Chemistry (journal)Powder diffractionIonCrystal structureCrystallographyNanotechnologyOptoelectronicsChemistry

Abstract

fetched live from OpenAlex

We report for the first time the synthesis of colloidal Ln3+/Yb3+ co-doped KY3F10nanocrystals (Ln = Er or Eu) viathermal decomposition. The transmission electron microscopy (TEM) studies indicated that the average size of the nanocrystals was approximately 15 nm. The nanocrystals crystallized in the cubic Fmm space group as confirmed by Rietveld refinement of the X-ray powder diffraction patterns and by electron diffraction analysis. The Eu3+ ion was used as a spectroscopic probe and its emission spectrum in colloidal KY3F10nanocrystals showed that the lanthanide ions replaces Y3+ in the lattice structure. When co-doped with Er3+/Yb3+, colloidal KY3F10nanocrystals exhibited visible (green and red) upconversion emissions following 978 nm excitation with a near-infrared (NIR) diode laser. Power dependence studies indicated that a two-photon energy transfer upconversion process was responsible for the NIR-to-visible upconversion.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.248
Teacher spread0.235 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations87
Published2009
Admission routes2
Has abstractyes

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