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Record W2044167837 · doi:10.1021/ma991974i

Domain Sizes Determination for Styrene−Isobutylene Block Copolymer Systems Using Solid-State NMR Spectroscopy

2000· article· en· W2044167837 on OpenAlexaff
Claudiu Neagu, Judit E. Puskás, M. A. Singh, Almeria Natansohn

Bibliographic record

VenueMacromolecules · 2000
Typearticle
Languageen
FieldChemistry
TopicAdvanced NMR Techniques and Applications
Canadian institutionsQueen's UniversityWestern University
FundersLaboratório Nacional de Luz Síncrotron
KeywordsCopolymerStyreneMaterials scienceIsobutyleneSmall-angle X-ray scatteringPhase (matter)Nuclear magnetic resonance spectroscopyPolymer chemistrySpectroscopyAnalytical Chemistry (journal)PolymerChemistryScatteringOrganic chemistryComposite material

Abstract

fetched live from OpenAlex

Solid-state NMR techniques were used to evaluate the sizes of the dispersed domains and the interface between the minor and the major phase in heterogeneous block copolymer systems with a relatively poor degree of ordering. Proton spin−lattice relaxation measurements and spin diffusion experiments were carried out on five samples of linear and star block copolymers of styrene, styrene- co -indene, and isobutylene. The morphology of the dispersed phase was considered cylindrical for all samples. The diameters of the dispersed cylinders were found to range between 7.9 and 48.5 nm for the linear samples and 22.6 nm for the star block copolymer sample. The thickness of the interface was estimated to be between 1.0 and 1.3 nm for all samples. SAXS measurements were employed to confirm the validity of the NMR data analysis.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.039
Threshold uncertainty score0.968

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.299
Teacher spread0.287 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations18
Published2000
Admission routes1
Has abstractyes

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