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Record W2051742393 · doi:10.1071/en04037

The Use of the ‘Ammonium Diffusion’ Method for d15N-NH4+ and d15N-NO3- Measurements: Comparison with Other Techniques

2004· article· en· W2051742393 on OpenAlexaff
Mathieu Sébilo, Bernhard Mayer, Micheline Grably, Daniel Billiou, André Mariotti

Bibliographic record

VenueEnvironmental Chemistry · 2004
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicGroundwater and Isotope Geochemistry
Canadian institutionsUniversity of Calgary
Fundersnot available
KeywordsAmmoniumChemistryContext (archaeology)NitrogenReproducibilityAqueous solutionDiffusionAmmonium nitrateAnalytical Chemistry (journal)Environmental chemistryInorganic chemistryChromatographyOrganic chemistry

Abstract

fetched live from OpenAlex

Environmental Context. Nitrogen is an essential element for all living organisms, and its biogeochemical cycle is connected to the cycling of carbon, sulfur, phosphorous, oxygen, and trace metals. Measurement of the isotopic composition of ammonium (NH4+) and nitrate (NO3-) containing samples provides a better understanding of the nitrogen cycle. While the established ‘ammonium diffusion’ measurement has many advantages, it is not easy for inexperienced people to prepare samples. This paper shows how the method can be simplified, ideally for samples freshly collected from the field. Abstract. Several methods have been developed for nitrogen isotope measurements on ammonium (NH4+) and nitrate (NO3-) in solid or aqueous samples. We have tested the accuracy and reproducibility of the ammonium diffusion method for d15N measurements on NH4+ and NO3- and compared this technique to other established methods. Our results show that the ammonium diffusion technique is capable of generating accurate and reproducible d15N values for minute quantities of NH4+-N and NO3--N in aqueous samples, if sufficient care is taken to minimize nitrogen blanks and to optimize the extraction procedure. Hence, the ammonium diffusion method offers an attractive alternative to more labour-intensive and costly methods for determining nitrogen isotope ratios of NH4+ and NO3- in aqueous samples.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.600
Threshold uncertainty score0.344

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.026
GPT teacher head0.214
Teacher spread0.188 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations85
Published2004
Admission routes1
Has abstractyes

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