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Record W2057389126 · doi:10.1002/qsar.200630037

A Quantitative Approach to the Estimation of Chemical Space from a Given Geometry by the Combination of Atomic Species

2007· article· en· W2057389126 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueQSAR & Combinatorial Science · 2007
Typearticle
Languageen
FieldComputer Science
TopicComputational Drug Discovery Methods
Canadian institutionsSickKids FoundationHospital for Sick Children
Fundersnot available
KeywordsMolecular geometryAtomic numberChemistryGeometrySpace (punctuation)Bond lengthComputational chemistryCrystallographyMoleculeMathematicsAtomic physicsPhysicsComputer scienceOrganic chemistryCrystal structure

Abstract

fetched live from OpenAlex

Abstract In order to estimate the size of chemical spaces, a quantitative approach was employed consisting of summing all possible combinations of atomic species generated computationally for a given three‐dimensional geometry. The atomic species were comprised of heavy atoms (N, C, O, S and Cl) and various numbers of H atoms ( e.g. , CH 3 and CH 2 groups). The assignment of atomic species to a given geometry maintained consistent bond orders between adjacent atoms. Between 10 8 and 10 19 compounds were generated from individual geometries. A slightly smaller number of compounds were obtained by applying a nonleadlikeness filter that considered the properties of the substituents. Principal component analysis using descriptors representing the molecular structures and properties revealed that the compounds generated from only one geometry largely covered the chemical space of known compounds. Moreover, the compounds with the best scores, defined as the interaction energies between the compounds and the protein, contained original ones within the entire collection of compounds generated from the same geometry. This method can be used to improve the scaffold of compound structures during drug development.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.004
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Theoretical or conceptual · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.737
Threshold uncertainty score0.434

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0040.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.003
Science and technology studies0.0000.001
Scholarly communication0.0000.001
Open science0.0020.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.304
Teacher spread0.281 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it