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Record W2057480901 · doi:10.1002/app.21175

Structure and ionic conductivity of a series of di‐<i>o</i>‐butyrylchitosan membranes

2004· article· en· W2057480901 on OpenAlex
Ying Wan, Katherine A. M. Creber, Brant A. Peppley, V. Tam Bui

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueJournal of Applied Polymer Science · 2004
Typearticle
Languageen
FieldEngineering
TopicFuel Cells and Related Materials
Canadian institutionsRoyal Military College of Canada
Fundersnot available
KeywordsMembraneCrystallinityChitosanThermogravimetric analysisPolymer chemistryThermal stabilityIonic conductivityIonic bondingConductivityDielectric spectroscopyMaterials scienceChemistryNuclear chemistryOrganic chemistryCrystallographyPhysical chemistryIonElectrolyteElectrochemistry

Abstract

fetched live from OpenAlex

Abstract Di‐ o ‐butyrylchitosan was prepared by reacting chitosan with butyric acid anhydride in the presence of perchloric acid as a catalyst. 13 C‐NMR and IR spectra of the modified chitosan suggested that both hydroxyl groups, at the C‐6 and C‐3 positions, in the chitosan molecules were substituted. The maximum degree of substitution was found to be less than 28%. The results of X‐ray diffractograms revealed that, in comparison with the unmodified chitosan membrane, the crystallinity of di‐ o ‐butyrylchitosan membranes was remarkably decreased. Meanwhile, it was also observed that the swelling indices of modified membranes were increased significantly in direct proportion to the degree of substitution. Thermogravimetric analysis indicated that the modified membranes exhibited a slightly increased thermal stability compared to the unmodified membrane. The ionic conductivity of di‐ o ‐butyrylchitosan membranes after hydration was investigated using impedance spectroscopy. Compared to the unmodified chitosan membrane, the hydrated di‐ o ‐butyrylchitosan membrane with a relatively high degree of the substitution showed an increased ionic conductivity of more than one order of magnitude. © 2004 Wiley Periodicals, Inc. J Appl Polym Sci 94: 2309–2323, 2004

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.006
Threshold uncertainty score0.271

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.185
Teacher spread0.181 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it