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Record W2059787490 · doi:10.1039/b406408a

Evaluation of the simultaneous use of standard additions and internal standards calibration techniques for inductively coupled plasma mass spectrometry

2004· article· en· W2059787490 on OpenAlexaff
Eric D. Salin, Margaret Antler, Guillaume Bort

Bibliographic record

VenueJournal of Analytical Atomic Spectrometry · 2004
Typearticle
Languageen
FieldChemistry
TopicMass Spectrometry Techniques and Applications
Canadian institutionsMcGill University
Fundersnot available
KeywordsInternal standardCalibrationStandard additionInductively coupled plasma mass spectrometryAnalytical Chemistry (journal)ChemistryInductively coupled plasmaThalliumMass spectrometryStandard solutionMatrix (chemical analysis)YttriumMolybdenumCobaltChromatographyPlasmaDetection limitInorganic chemistry

Abstract

fetched live from OpenAlex

The use of internal standards combined with standard additions calibration for inductively coupled plasma mass spectrometry (ICP-MS) is discussed. Yttrium, rhodium, magnesium, cobalt, copper, nickel, silver, thallium, molybdenum and lead were analyzed in solutions of known composition with a 500 mg ml−1 Na matrix. Additionally, the Mg, Co, Y, Rh and Pb signals were used as internal standards for the other elements in the same matrix. Severe drift effects were simulated by drastically altering the liquid sample uptake rate. The signals were used to compare the results obtained using four different calibration methods: external standards, standard additions, internal standards and standard additions in combination with an internal standard. The average errors for external standards varied from 23 to 41% while the average errors for internal standards ranged from 1 to 71%. The error for standard additions was 45%. The use of standard additions with an internal standard produced an average error of 0.7–5%, suggesting that this is a powerful calibration technique.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.082
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.002
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.024
GPT teacher head0.308
Teacher spread0.284 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations23
Published2004
Admission routes1
Has abstractyes

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