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Record W2060302835 · doi:10.1002/aic.10039

On the activity of ions and the junction potential: Revised values for all data

2004· article· en· W2060302835 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueAIChE Journal · 2004
Typearticle
Languageen
FieldChemical Engineering
TopicChemical and Physical Properties in Aqueous Solutions
Canadian institutionsMcGill University
FundersNatural Sciences and Engineering Research Council of CanadaXunta de Galicia
KeywordsIonElectrolyteWork (physics)CalibrationSign (mathematics)Interpretation (philosophy)ThermodynamicsChemistryActivity coefficientElectrodeStatistical physicsMathematicsPhysicsMathematical analysisStatisticsPhysical chemistryComputer science

Abstract

fetched live from OpenAlex

Abstract This work presents an in‐depth study of the interrelation between the junction potential E J and the activity of individual ions. The need to correct for the sign of the junction potential employed in previous publications is used to confirm that the calibration of the ion‐selective electrodes largely cancels errors in the estimation of E J . Revised values of the activity coefficients of individual ions are presented for all systems previously measured. A rederivation of Henderson equation is used to clarify the interpretation of its terms for asymmetric electrolytes. A new analytical equation to calculate E J is derived and tested. This equation corrects for the nonideality of solutions and for the concentration dependence of the conductivity. The correction for nonideality is only necessary for the ions present in both the sample and the reference electrode solutions. The new equation represents a major improvement over the Henderson equation for E J calculations. © 2004 American Institute of Chemical Engineers AIChE J, 50: 445–462, 2004

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.731
Threshold uncertainty score0.168

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.043
GPT teacher head0.274
Teacher spread0.230 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it