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Record W2062175990 · doi:10.1021/es048502q

Continuous Fermentative Hydrogen Production Using a Two-Phase Reactor System with Recycle

2005· article· en· W2062175990 on OpenAlexaff
Jeremy Kraemer, David M. Bagley

Bibliographic record

VenueEnvironmental Science & Technology · 2005
Typearticle
Languageen
FieldEngineering
TopicAnaerobic Digestion and Biogas Production
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsMethanogenesisChemistryChemical oxygen demandAcidogenesisEffluentHydraulic retention timeHydrogen productionAlkalinityPulp and paper industryMethaneHydrogenFermentative hydrogen productionChemostatAnaerobic digestionWastewaterEnvironmental engineeringEnvironmental scienceOrganic chemistryBacteria

Abstract

fetched live from OpenAlex

The effects of effluent recycle were examined in a two-phase anaerobic system where the first phase was operated for fermentative hydrogen production and the second for methanogenesis. The hydrogen reactor was operated as a chemostat at 35 degrees C and pH 5.5 with a 10 h hydraulic retention time, and the methane reactor was operated as an up-flow reactor at 28 degrees C and pH between 6.9 and 7.2. Two recycle ratios were examined: 0 and 0.98. Effluent recycle reduced the required alkalinity for pH control by approximately 40%. The H2 productivity metric, with a basis in electrons and incorporating both gaseous and dissolved H2, was developed as a more fundamental reporting method than the molar H2 yield. Without recycle, the H2 productivity was 0.115 g of H2 COD/g of feed COD, but decreased to 0.015 q of H2 COD/g of feed COD with recycle (COD = chemical oxygen demand). Mass balances indicated the lower H2 productivity during recycle was due to electrons being partitioned to methane and less-oxidized soluble constituents such as propionic acid, ethanol, and butanol. The results indicated that achieving high H2 productivity with nonsterile wastewaters will be challenging and membrane filtration of the recycle liquid may be required to exclude the return of hydrogen-consuming organisms.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0010.001
Open science0.0020.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.223
Teacher spread0.216 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations121
Published2005
Admission routes1
Has abstractyes

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