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Record W2065257155 · doi:10.1063/1.1518683

A revised experimental absolute magnetic shielding scale for oxygen

2002· article· en· W2065257155 on OpenAlexafffund
Roderick E. Wasylishen, David L. Bryce

Bibliographic record

VenueThe Journal of Chemical Physics · 2002
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicAtmospheric Ozone and Climate
Canadian institutionsUniversity of Alberta
FundersNatural Sciences and Engineering Research Council of CanadaCanada Research ChairsUniversity of Alberta
KeywordsElectromagnetic shieldingOxygenChemistryIsotropyCarbon monoxideMonoxideAnalytical Chemistry (journal)Ab initioConstant (computer programming)Ab initio quantum chemistry methodsAbsolute scaleAtomic physicsNuclear magnetic resonanceMaterials sciencePhysicsMoleculeInorganic chemistryOptics

Abstract

fetched live from OpenAlex

A revised absolute magnetic shielding scale for oxygen is established based on a recently reported highly precise experimental measurement of the O17 spin-rotation constant in carbon monoxide. The isotropic oxygen magnetic shielding constant for C12O17 at the equilibrium geometry, σe, is found to be −56.8±0.6 ppm. The experimental rovibrationally averaged value of the shielding constant at 300 K, 〈σ〉300 K, is −62.7±0.6 ppm, in excellent agreement with the ab initio value reported by Vaara et al. [J. Chem. Phys. 109, 8388 (1998)]. Based on the revised scale and on experimentally known oxygen chemical shifts, 〈σ〉300 K (H2O(l)) is 287.5±0.6 ppm and 〈σ〉300 K (H2O(g)) is 323.6±0.6 ppm.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.248
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.022
GPT teacher head0.224
Teacher spread0.202 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations116
Published2002
Admission routes2
Has abstractyes

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