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Record W2065349798 · doi:10.1021/es803138z

Multiyear Total and Methyl Mercury Exports from Two Major Sub-Arctic Rivers Draining into Hudson Bay, Canada

2009· article· en· W2065349798 on OpenAlexaffabout
Jane L. Kirk, Vincent L. St. Louis

Bibliographic record

VenueEnvironmental Science & Technology · 2009
Typearticle
Languageen
FieldEnvironmental Science
TopicMercury impact and mitigation studies
Canadian institutionsUniversity of Alberta
Fundersnot available
KeywordsBayMercury (programming language)MethylmercuryEstuaryArcticHydrology (agriculture)Environmental scienceOceanographyDissolved organic carbonWetlandEnvironmental chemistryGeologyChemistryEcologyBioaccumulation

Abstract

fetched live from OpenAlex

From 2003 to 2007, concentrations of total mercury and methylmercury (THg and MeHg) were continuously measured in two Canadian sub-Arctic rivers (the Nelson and the Churchill) that drain into western Hudson Bay. THg and MeHg concentrations were low in the Nelson River (mean i standard deviation, 0.88 +/- 0.33 and 0.05 +/- 0.03 ng L(-1), respectively). The Churchill River, however, had high concentrations of Hg, particularly MeHg (1.96 +/- 0.8 and 0.18 +/- 0.09 ng L(-1), respectively) and hence may be an important source of MeHg to organisms feeding in the Churchill River estuary. A large portion of THg in the Nelson River was particulate-bound (39 +/- 23%), while in the Churchill River, most was in the dissolved form (78 +/- 15%) and is likely dissolved organic carbon (DC)-bound Hg originating in the surrounding wetlands. In fact, both the Nelson and Churchill Rivers had high DOC concentrations and were therefore large exporters of DOC to Hudson Bay (1480 +/- 723 and 392 +/- 309 x 10(3) t year(-1), respectively) compared to rivers to the south and east Despite high Churchill River Hg concentrations, due to large Nelson River flows, average THg and MeHg exports to Hudson Bay from the Churchill River (37 +/- 28 and 4 +/- 4 kg year(-1), respectively) were about one-third and half the Nelson River exports (113 +/- 52 and 9 +/- 4 kg year(-1)). Interestingly, combined Hg exports to Hudson Bay from Nelson and Churchill River discharge are comparable to THg inputs from Hudson Bay springtime snowmelt (177 +/-140 kg year(-1)) but are approximately 13 times greater than MeHg snowmelt inputs (1 +/- 1 kg year(-1)). Although Hg inputs from rivers and snowmelt together may account for a large portion of the THg pool in Hudson Bay, these inputs account for a lesser portion of the MeHg pool, thus highlighting the importance of water column Hg(ll) methylation as a source of MeHg to Hudson Bay marine food webs.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.599
Threshold uncertainty score0.987

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0010.002
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.222
Teacher spread0.217 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations62
Published2009
Admission routes2
Has abstractyes

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