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Record W2065786632 · doi:10.1021/es071819g

Occurrence and Biomagnification of Polychlorinated Naphthalenes and Non- and Mono-<i>ortho</i> PCBs in Lake Ontario Sediment and Biota

2008· article· en· W2065786632 on OpenAlexaffabout
Paul A. Helm, Sarah B. Gewurtz, D. Michael Whittle, Chris Marvin, Aaron T. Fisk, Gregg T. Tomy

Bibliographic record

VenueEnvironmental Science & Technology · 2008
Typearticle
Languageen
FieldEnvironmental Science
TopicToxic Organic Pollutants Impact
Canadian institutionsEnvironment and Climate Change CanadaMinistry of the Environment, Conservation and Parks
Fundersnot available
KeywordsBiomagnificationBioaccumulationCongenerEnvironmental chemistryBiotaBenthic zoneTroutTrophic levelDry weightPersistent organic pollutantBioconcentrationChemistryPolychlorinated biphenylSedimentEnvironmental scienceEcologyPollutantBiologyFisheryFish <Actinopterygii>

Abstract

fetched live from OpenAlex

Biota and surface sediments collected from Lake Ontario were analyzed for polychlorinated naphthalenes (PCNs) and non- and mono-ortho-substituted polychlorinated biphenyls (n/ m-o-PCBs) to compare bioaccumulation behavior of these classes of dioxin-like chemicals in a food web from the Great Lakes. Mean sigmaPCN concentrations (tri-octaCN) ranged from 14 +/- 9 pg/g in plankton to 3500 +/- 3200 pg/g (wet weight) in lake trout while sediments contained from 21 to 38 ng/g (dry weight). Principal components analysis of PCN congener patterns indicated that chlorine substitution determined which congeners favored accumulation (e.g., CN-42, -52, -60, -66, -67, and -73), while others may be subject to metabolism. The bioaccumulative congeners exhibited similar trophic magnification factors (TMFs; 1.23-1.42) and biomagnification factors (BMFs; 5.5-8.6) to the n/m-o-PCBs for the trout/weighted diet relation, although BMFs for a benthic feeding relationship (slimy sculpin/Diporeia) indicated that the n/m-o-PCBs were more bioavailablethroughthe benthic pathway. PCNs contribute significantly to the burden of dioxin-like compounds in Lake Ontario biota, contributing between 12 and 22% of total PCN + PCB TEQ in lake trout and up to 69% in benthic organisms.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesScience and technology studies
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.262
Threshold uncertainty score0.997

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.006
Scholarly communication0.0000.000
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.200
Teacher spread0.193 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations102
Published2008
Admission routes2
Has abstractyes

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