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Record W2069886864 · doi:10.1021/ie5004027

Characterization and Inhibition of a Nickel-Alpha-Hydroxyoxime (LIX 63) Salt Precipitate Formed under Proposed Commercial Operating Conditions

2014· article· en· W2069886864 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2014
Typearticle
Languageen
FieldEngineering
TopicExtraction and Separation Processes
Canadian institutionsTeck (Canada)
Fundersnot available
KeywordsNickelChemistryInorganic chemistrySalt (chemistry)PrecipitationSulfuric acidSulfateCobaltManganeseNitrateMagnesiumSolventAqueous solutionNuclear chemistryOrganic chemistry

Abstract

fetched live from OpenAlex

As a prospective commercial solvent extraction (SX) process, laboratory-scale continuous tests were recently undertaken to assess the use of a solution of LIX 63 hydroxyoxime (“hydroxyoxime”) and Versatic 10 to kinetically separate cobalt from a nickel-rich sulfate solution while simultaneously rejecting manganese and magnesium. A material quantity of blue precipitate observed in the strip stage cells during decommissioning has been identified as the sulfate salt of the nickel-tris hydroxyoxime complex. As precipitation during SX is undesirable, the effect of various operating parameters on precipitate formation has been investigated. Minimizing aqueous nickel and/or sulfuric acid concentration and/or increasing organic polarity can overcome this problem. Where it forms, hydroxyoxime and nickel can be recovered from the precipitate by redissolution under suitable (e.g., low acid) operating conditions. The nitrate salt counterpart of this sulfate precipitate has been crystallographically characterized using a short chained (C 8 ) analogue of LIX 63 hydroxyoxime, revealing the coordination of three neutral hydroxyoxime ligands around nickel, forming a monomeric coordination complex cation counterbalanced by nitrate anions.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.057
Threshold uncertainty score0.781

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.057
GPT teacher head0.318
Teacher spread0.260 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it