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Record W2070809805 · doi:10.1021/ef900269q

A Comprehensive Analysis of Organic Matter Removal from Clay-Sized Minerals Extracted from Oil Sands Using Low Temperature Ashing and Hydrogen Peroxide

2009· article· en· W2070809805 on OpenAlexaff
Adebukola Adegoroye, Peter Uhlík, Oladipo Omotoso, Zhenghe Xu, Jacob H. Masliyah

Bibliographic record

VenueEnergy & Fuels · 2009
Typearticle
Languageen
FieldChemistry
TopicPetroleum Processing and Analysis
Canadian institutionsDevon Energy (Canada)
Fundersnot available
KeywordsSideriteOil sandsTailingsOrganic matterClay mineralsChemistryHydrogen peroxideAdsorptionEnvironmental chemistryAshingAsphaltMineralogyMaterials sciencePyriteOrganic chemistry

Abstract

fetched live from OpenAlex

Understanding mineralogy and surface properties of clays is very vital in oil sands processing and tailings management. Clay-sized minerals (CSM) in oil sands are often contaminated by tightly adsorbed organics during hydrocarbon removal, thereby increasing surface hydrophobicity and making characterization of CSM problematic. This study evaluates the use of low temperature ashing (LTA) and hydrogen peroxide (H 2 O 2 ) for the removal of adsorbed organic matter (OM) from CSM without changing its mineralogy. CSM isolated from tailings and bitumen froth of a Denver flotation cell after oil sands extraction was treated by H 2 O 2 and LTA. Both techniques were found to be effective in removing OM from the CSM as shown by the infrared spectra of the samples. The wettability of the CSM increased with treatment. Elemental analysis showed a reduction in carbon, hydrogen, and nitrogen. Infrared band for siderite at 864 cm −1 was observed for the isolated and LTA-treated CSM but was absent for those treated by H 2 O 2 . The absence of siderite in the X-ray diffraction patterns of the H 2 O 2 -treated CSM further substantiates its oxidation by H 2 O 2 . Cation exchange capacity of model clays and samples was found to be unaffected by LTA treatment, unlike those treated with H 2 O 2 . Overall, LTA appears to be a more suitable method than H 2 O 2 for organic matter removal from the isolated CSM because of its selectivity for decomposing only organics.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.229
Teacher spread0.219 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations12
Published2009
Admission routes1
Has abstractyes

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