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First-principles calculation on the Curie temperature of Gd<sub>3</sub>NiSi<sub>2</sub>

2009· article· en· W2072116974 on OpenAlexaff
Xubo Liu, Z. Altounian

Bibliographic record

VenueJournal of Physics Condensed Matter · 2009
Typearticle
Languageen
FieldMaterials Science
TopicMagnetic and transport properties of perovskites and related materials
Canadian institutionsMcGill University
Fundersnot available
KeywordsCondensed matter physicsCurie temperatureMagnetic momentMagnetizationLocal-density approximationCoherent potential approximationSpin (aerodynamics)Electronic structureCurieCoupling (piping)Fermi levelDensity of statesDensity functional theoryFormula unitElectronic band structureChemistryPhysicsMaterials scienceMagnetic fieldFerromagnetismQuantum mechanicsComputational chemistryCrystal structureThermodynamicsCrystallography

Abstract

fetched live from OpenAlex

The electronic structure and magnetic properties for Gd(3)NiSi(2) have been studied theoretically from a first-principles density functional calculation. The energy band structure is calculated in a local spin density approximation (LSDA), and in a LSDA+Hubbard U approach (LSDA+U), respectively. For Gd atoms, in the LSDA+U approximation, seven spin-up 4f bands are fully occupied and situated at the bottom of Si s states, while the spin-down 4f hole levels are completely unoccupied and well above the Fermi level. The calculated magnetic moments for the three Gd sites vary from 7.13 to 7.16 µ(B), leading to a total magnetization of 21.5 µ(B) per formula unit including the small induced moments at Ni and Si atoms. The exchange coupling parameters for the nearest Gd-Gd pairs (J(Gd-Gd)) are 0.16 mRyd, 0.14 mRyd and 0.19 mRyd in the three Gd sub-lattices, respectively. The inter-site distance dependence of J(Gd-Gd) shows a RKKY-like oscillation. The estimated Curie temperature is about 251 K from the calculated exchange coupling parameters based on the mean-field approximation, in good agreement with the experimental value (T(C)(exp.) = 215 K).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.010
Threshold uncertainty score0.019

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.001
Science and technology studies0.0010.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0040.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.205
Teacher spread0.192 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations5
Published2009
Admission routes1
Has abstractyes

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