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Record W2072636575 · doi:10.1021/ef030156v

Colloidal Properties of Bio-oils Obtained by Vacuum Pyrolysis of Softwood Bark:  Aging and Thermal Stability

2004· article· en· W2072636575 on OpenAlexaff
Abdelkader Chaala, Tuya Ba, Manuel Garcı̀a-Pèrez, Christian Roy

Bibliographic record

VenueEnergy & Fuels · 2004
Typearticle
Languageen
FieldEngineering
TopicThermochemical Biomass Conversion Processes
Canadian institutionsUniversité Laval
Fundersnot available
KeywordsPyrolysisThermogravimetrySoftwoodDifferential scanning calorimetryRheologyPyrolysis oilMaterials scienceThermal stabilityChemistryChemical engineeringComposite materialOrganic chemistry

Abstract

fetched live from OpenAlex

The objective of this study is to provide background information on pyrolysis oil for gas turbine applications. The bio-oil investigated consists of an upper layer and a bottom layer. It has been produced by vacuum pyrolysis of softwood bark. The storage stability and the thermal behavior of the whole bio-oil, the upper layer, and the bottom layer were evaluated. The samples were stored at different temperatures (40, 50, and 80 °C) for up to 168 h and at room temperature for up to 1 year. Morphology, rheology, thermogravimetry, and differential scanning calorimetry tests were performed on the bio-oil samples after their aging. The results indicated that the properties of the whole bio-oil are significantly altered when the bio-oil was heated at 80 °C, whatever the range of time investigated. The impact after heating to 50 °C was not critical for storage and handling purposes however, as shown by a series of rheological data. It was found that the aging effect is more pronounced for the bottom layer than for the upper layer. The presence of the upper layer reduced the aging rate of the bio-oil as a whole. The molecular weight increase after heating the whole bio-oil for 1 week at 80°C was equivalent to keeping the sample for 1 year at room temperature. This increase was mainly caused by polymerization of the bottom-layer-contained compounds. Aging of the raw bio-oil at room temperature resulted in a dramatic viscosity increase during the first 60 days, after which a plateau was reached.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.589

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.173
Teacher spread0.166 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations73
Published2004
Admission routes1
Has abstractyes

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