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Record W2075593175 · doi:10.1002/pen.11075

Polymerization compounding: Epoxy‐montmorillonite nanocomposites

2002· article· en· W2075593175 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenuePolymer Engineering and Science · 2002
Typearticle
Languageen
FieldMaterials Science
TopicPolymer Nanocomposites and Properties
Canadian institutionsUniversité Laval
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsOrganoclayMaterials scienceThermogravimetric analysisDifferential scanning calorimetryGlass transitionNanocompositeMontmorilloniteDynamic mechanical analysisEpoxyFourier transform infrared spectroscopyComposite materialIn situ polymerizationCuring (chemistry)PolymerizationPolymer chemistryChemical engineeringPolymer

Abstract

fetched live from OpenAlex

Abstract A strategy to design intercalated montmorillonite nanocomposites has been explored. A commercial organoclay, 1.34 TCN (Nanocor Inc.), with bis(2‐hydroxylethy1) methy1 tallow ammonium, was modified by tolylene 2,4‐diisocyanate (TDI) and bisphenol A (BA). Thermogravimetric analysis (TGA), Fourier transform infrared (FTIR) spectroscopy and X‐ray diffraction (XRD) results of unmodified and modified 1.34 TCN (1.34‐TDI‐BA) indicate that TDI and BA have reacted with hydroxy1 groups on the surface of 1.34 TCN and hydroxy1 groups in the interlayer of 1.34 TCN. Using a classical two‐stage cure process with diamine as curing agent, intercalated epoxy nanocomposites were prepared for both types of organoclays. XRD and TEM results showed that the basal spacing of clay in nanocomposites was 3.68 and 4.42 nm for 1.34 TCN and 1.34‐TDI‐BA, respectively. Dynamic mechanical analysis (DMA) was performed on both modified and unmodified organoclay composites. Modified organoclay composites were found to have enhanced storage moduli, particularly at temperatures higher than the glass transition, T g , of the matrix. Glass transition temperatures extracted from linear viscoelastic data are found to be slightly higher for modified organoclay nanocomposites, indicating enhanced interactions between the modified organoclay and the epoxy matrix. These results were also confirmed by independent measurements of T g using differential scanning calorimetry (DSC).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.037
Threshold uncertainty score0.702

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.195
Teacher spread0.183 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it