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Record W2075698096 · doi:10.1021/ie901861y

Fischer−Tropsch Synthesis in a Slurry Reactor Using a Nanoiron Carbide Catalyst Produced by a Plasma Spray Technique

2010· article· en· W2075698096 on OpenAlexafffund
Jasmin Blanchard, Nicolas Abatzoglou, Roham Eslahpazir-Esfandabadi, F. Gitzhofer

Bibliographic record

VenueIndustrial & Engineering Chemistry Research · 2010
Typearticle
Languageen
FieldChemical Engineering
TopicCatalysts for Methane Reforming
Canadian institutionsUniversité de Sherbrooke
FundersNatural Resources CanadaNatural Sciences and Engineering Research Council of Canada
KeywordsFischer–Tropsch processSlurryCatalysisCarbideChemical engineeringMaterials scienceSyngasChemistryMetallurgyOrganic chemistryEngineeringComposite material

Abstract

fetched live from OpenAlex

A new catalyst, composed of iron carbide nanoparticles (FeCNPs) and synthesized by plasma-spraying technology, was tested for Fischer−Tropsch synthesis (FTS) in a continuously stirred slurry reactor. The plasma-produced FeCNPs were core−matrix structures (FeC-rich core inside a graphitic carbon matrix) which protected air-sensitive carbides, preventing oxidation during their handling. The reactant used for FTS testing was simulated syngas with a composition similar to that obtained from air gasification of urban waste. This work reports the optimization of a new nanocatalyst reduction/activation protocol aimed at maximizing catalyst activity and a 100-h-long test performed to examine the catalyst’s behavior over time. The catalyst was compared with Nanocat commercial nanoiron powder, and the results showed that its activity and robustness were higher. Conversion with the Nanocat catalyst was slightly but not statistically significantly lower than with the plasma-produced catalyst. However, 6% CH 4 selectivity with the plasma-produced catalyst was significantly lower than the 10% obtained with Nanocat.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.054
GPT teacher head0.313
Teacher spread0.260 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations33
Published2010
Admission routes2
Has abstractyes

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