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Record W2075973187 · doi:10.1139/p11-082

Self-compressed inhomogeneous stabilized jellium model and surface relaxation of simple metal thin films

2011· article· en· W2075973187 on OpenAlexvenueno aff

Bibliographic record

VenueCanadian Journal of Physics · 2011
Typearticle
Languageen
FieldChemistry
TopicAdvanced Physical and Chemical Molecular Interactions
Canadian institutionsnot available
Fundersnot available
KeywordsJelliumIonic bondingSlabElectron densityRelaxation (psychology)Work (physics)Surface (topology)Thin filmMetal

Abstract

fetched live from OpenAlex

The interlayer spacing near the surface of a crystal is different from that of the bulk. As a result, the value of the ionic density in the normal direction and near to the surface shows some variation from the bulk value, which is oscillatory in shape. To describe this behavior simply, we have formulated the self-compressed inhomogeneous stabilized jellium model and have applied it to simple metal thin films. In this model, for a ν-layered slab, each ionic layer is replaced by a jellium slice of constant density. The equilibrium densities of the slices are determined by minimizing the total energy per electron of the slab with respect to the slice densities. However, to avoid the complications that arise because of the increasing number of independent slice-density parameters for large-ν slabs, we consider a simplified version of the model that consists of only three jellium slices: one inner bulk slice with density [Formula: see text] and two similar surface slices, each of density [Formula: see text]. In this simplified model, each slice may contain more than one ionic layer. Application of this model to ν-layered slabs (3 ≤ ν ≤ 10) of Al, Na, and Cs shows that, in the equilibrium state, [Formula: see text] differs from [Formula: see text]. The difference is significant in the Al case, and the slab is more stable than that predicted by the homogeneous model with only one density parameter for the whole jellium background. In addition, we have calculated the overall relaxations, the work functions, and the surface energies and compared them with the results of earlier works.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.032
Threshold uncertainty score0.419

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.221
Teacher spread0.202 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2011
Admission routes1
Has abstractyes

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