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Record W2077804561 · doi:10.1021/ma011227x

Preparation and Characterization of Poly[2,3-dimethyl-1-(4-thien-3-ylbenzyl)-1<i>H</i>-imidazol-3-ium] Bis((trifluoromethyl)sulfonyl)imide

2002· article· en· W2077804561 on OpenAlexaff
Éric Naudin, Hoang Anh Ho, Marc‐André Bonin, Livain Breau, Daniel Bélanger

Bibliographic record

VenueMacromolecules · 2002
Typearticle
Languageen
FieldMaterials Science
TopicConducting polymers and applications
Canadian institutionsUniversité du Québec à Montréal
Fundersnot available
KeywordsChemistryTrifluoromethylImideSulfonylDichloromethaneBromideThiopheneCationic polymerizationPolymer chemistryRedoxIonic liquidMonomerElectrochemistryPolymerMedicinal chemistryOrganic chemistryPhysical chemistryCatalysisElectrodeSolvent

Abstract

fetched live from OpenAlex

A new 3-fluorophenylthiophene derivative bearing a cationic imidazolium group in the para position of the phenyl ring was synthesized by a multistep procedure which involves, in a key step, the reaction of 3-[4-(bromomethyl)phenyl]thiophene with 1,2-dimethylimidazole. The bis[(trifluoromethyl)sulfonyl]imide (TFSI) salt was obtained by anion exchange of the imidazolium bromide precursor with LiTFSI. The electrochemical oxidation of the title monomer in dichloromethane afforded an electronically conducting polymer displaying both p- and n-doping redox waves. These redox processes were also accompanied by change in absorption spectra that confirmed the modification of the electronic properties of the polymer upon both p- and n-doping.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.008
Threshold uncertainty score0.864

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.019
GPT teacher head0.257
Teacher spread0.239 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2002
Admission routes1
Has abstractyes

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