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Record W2079650151 · doi:10.1029/2003jb002659

Effect of pressure on liquid‐liquid miscibility gaps: A case study of the systems CaO‐SiO<sub>2</sub>, MgO‐SiO<sub>2</sub>, and CaMgSi<sub>2</sub>O<sub>6</sub>‐SiO<sub>2</sub>

2004· article· en· W2079650151 on OpenAlexaff
Pierre Hudon, In‐Ho Jung, Don R. Baker

Bibliographic record

VenueJournal of Geophysical Research Atmospheres · 2004
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicGeological and Geochemical Analysis
Canadian institutionsPolytechnique MontréalMcGill University
Fundersnot available
KeywordsMiscibilityIonic radiusSpinodal decompositionMetastabilityMaterials sciencePhase diagramPhase (matter)Atmospheric pressureThermodynamicsIonChemistryGeologyOrganic chemistryPolymerPhysics

Abstract

fetched live from OpenAlex

In order to investigate the effects of liquid‐liquid phase separation on the igneous evolution of planetary bodies, we investigated immiscibility in the systems CaO‐SiO2, MgO‐SiO2, and CaMgSi2O6‐SiO2 at pressures to 1.5 GPa. Few changes are observed in the size of the miscibility gaps in these systems at 1.0 GPa. The decrease of the stable area of the gaps is mainly due to the increase of the monotectic temperature because the latter closely follows the melting temperature of SiO2 at high pressure. The pressure at which the whole CaO‐MgO‐SiO2 miscibility gap becomes metastable is estimated to be 1.81 GPa. The thermal and compositional extents of miscibility gaps associated with network‐modifier cations (such as Ca2+) do not change significantly with increasing pressure, but the extents are increased for amphoteric cations (such as Mg2+), and the change is more pronounced if the latter have small ionic radii and high ionic potentials. Cations possessing high crystal field stabilization energies produce the largest immiscibility fields at atmospheric pressure, and the passage from the high‐spin to the low‐spin state with increasing pressure is expected to yield even larger miscibility gaps. Magmas containing substantial amounts of amphoteric cations and cations with high crystal field stabilization energies are therefore potential candidates to develop immiscibility at high pressures.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0010.001
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.017
GPT teacher head0.266
Teacher spread0.250 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations16
Published2004
Admission routes1
Has abstractyes

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