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Record W2081340016 · doi:10.1021/es062647a

Time-Weighted Average Water Sampling in Lake Ontario with Solid-Phase Microextraction Passive Samplers

2007· article· en· W2081340016 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.
aboutThe title or abstract carries a Canadian signal from the geographic lexicon.

Bibliographic record

VenueEnvironmental Science & Technology · 2007
Typearticle
Languageen
FieldChemistry
TopicAnalytical chemistry methods development
Canadian institutionsUniversity of WaterlooEnvironment and Climate Change Canada
FundersNatural Sciences and Engineering Research Council of CanadaGuangdong Provincial Key Laboratory of Environmental Pollution Control and Remediation Technology
KeywordsSolid-phase microextractionPolydimethylsiloxaneSampling (signal processing)Environmental scienceChromatographyDetection limitExtraction (chemistry)PollutantEnvironmental chemistryVolume (thermodynamics)Gas chromatographyAnalyteChemistryAnalytical Chemistry (journal)Gas chromatography–mass spectrometryMass spectrometry

Abstract

fetched live from OpenAlex

In this study, three types of solid-phase microextraction (SPME) passive samplers, including a fiber-retracted device, a polydimethylsiloxane (PDMS)-rod and a PDMS-membrane, were evaluated to determine the time weighted average (TWA) concentrations of polycyclic aromatic hydrocarbons (PAHs) in Hamilton Harbor (the western tip of Lake Ontario, ON, Canada). Field trials demonstrated that these types of SPME samplers are suitable for the long-term monitoring of organic pollutants in water. These samplers possess all of the advantages of SPME: they are solvent-free, sampling, extraction and concentration are combined into one step, and they can be directly injected into a gas chromatograph (GC) for analysis without further treatment. These samplers also address the additional needs of a passive sampling technique: they are economical, easy to deploy, and the TWA concentrations of target analytes can be obtained with one sampler. Moreover, the mass uptake of these samplers is independent of the face velocity, or the effect can be calibrated, which is desirable for long-term field sampling, especially when the convection conditions of the sampling environment are difficult to measure and calibrate. Among the three types of SPME samplers that were tested, the PDMS-membrane possesses the highest surface-to-volume ratio, which results in the highest sensitivity and mass uptake and the lowest detection level.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.011
Threshold uncertainty score0.996

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.002
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0050.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.279
Teacher spread0.267 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it