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Solvent and pH resistance of surface crosslinked chitosan/poly(acrylonitrile) composite nanofiltration membranes

2000· article· en· W2081378917 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueJournal of Applied Polymer Science · 2000
Typearticle
Languageen
FieldEnvironmental Science
TopicMembrane Separation Technologies
Canadian institutionsNational Research Council Canada
Fundersnot available
KeywordsMembranePermeationGlutaraldehydeSolventSwellingAcrylonitrileChemistrySolubilityNanofiltrationPolymer chemistryHildebrand solubility parameterAqueous solutionChemical engineeringNuclear chemistryChromatographyPolymerOrganic chemistryCopolymer

Abstract

fetched live from OpenAlex

The resistance of novel surface crosslinked Chitosan/poly(acrylonitrile) (PAN) composite nanofiltration (NF) membranes to pH and organic solvents was studied with respect to the effects of crosslinking parameters, namely, glutaraldehyde concentration and crosslinking time. The pH resistance was determined by permeation of aqueous acidic (pH 2.5) and basic (pH 11) solutions as well as swelling studies in the pH range of 2.5–11. The solvent resistance was determined by swelling, immersion, and permeation studies with several industrially important organic solvents, namely methanol, ethanol, iso-propanol, methyl ethyl ketone, ethyl acetate and hexane. It was observed that the crosslinked composite membranes maintain the permeate fluxes for test solvents for 2 h of continuous operation without any significant change in flux. SEM studies on membrane samples after immersion as well as permeation with the above-mentioned solvents indicated that the membrane morphology was maintained. The results are explained in terms of solvent–membrane polar and hydrophobic interactions, using solubility parameters of membrane and solvents and dielectric constants of solvents. Pure water flux and polyethylene glycol transmission data indicated that at pH 2.5 and 11, the membrane stability increased with increasing glutaraldehyde concentration and was much better at pH 11 than at pH 2.5. All surface crosslinked membranes showed reduced swelling between pH 4–10. © 2000 John Wiley & Sons, Inc. J Appl Polym Sci 77: 1782–1793, 2000

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.013
Threshold uncertainty score0.646

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.002
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.231
Teacher spread0.223 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it