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Record W2092582826 · doi:10.1002/app.32189

Color improvment of C<sub>9</sub>hydrocarbon resin by hydrogenation over 2% Pd/γ‐alumina catalyst: Effect of degree of aromatic rings hydrogenation

2010· article· en· W2092582826 on OpenAlexaff
Nikom Sae‐Ma, Piyasan Praserthdam, Joongjai Panpranot, Somboon Chaemchuen, Siraprpha Dokjamp, Kongkiat Suriye, Garry L. Rempel

Bibliographic record

VenueJournal of Applied Polymer Science · 2010
Typearticle
Languageen
FieldChemistry
TopicMetal-Organic Frameworks: Synthesis and Applications
Canadian institutionsUniversity of Waterloo
Fundersnot available
KeywordsAlicyclic compoundChemistryAromaticityAromatic hydrocarbonFourier transform infrared spectroscopyCatalysisHydrocarbonNuclear chemistryOrganic chemistryPolymer chemistryMoleculeChemical engineering

Abstract

fetched live from OpenAlex

Abstract Color improvement of commercial C 9 hydrocarbon resin (c‐C 9 HR) and prepared C 9 hydrocarbon resin (p‐C 9 HR) has been investigated under various hydrogenation conditions over 2% Pd/γ‐alumina catalysts. The degrees of aromatic rings hydrogenation (DHs) and molecular structure of resin were determined from nuclear magnetic resonance of 1 H and 13 C ( 1 H‐NMR and 13 C‐NMR) and Fourier transform infrared spectroscopy (FTIR) analyses. The starting c‐C 9 HR presented in yellow color (Gardner color No. 8.4). Under the hydrogenation conditions used (H 2 pressure 70 bar, 250°C, and 8 h), the ethylenic proton in c‐C 9 HR was completely removed, but the aromatic rings content remained unaltered and very little change in resin color was observed (Gardner color No.8.1). On the other hand, the starting p‐C 9 HR contained only unsaturated aromatic proton with Gardner color No.17.1. Under similar conditions, aromatic rings in p‐C 9 HR were converted to alicyclic rings, and its color was reduced to Gardner color No.5.7. By varying the DH of aromatics in p‐C 9 HR, two‐step decolorization was observed in which at lower DH (≤10%) the color decreased sharply from 17.1 to 9.3, while further color reduction to 5.7 was obtained when the DH was increased to 94%. It is suggested that both color body and aromatic rings were the main sources contributing to C 9 HR color. Nevertheless, color stability of the resin during heat treatment was significantly improved by hydrogenation especially at DH ≥ 50%. © 2010 Wiley Periodicals, Inc. J Appl Polym Sci, 2010

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.009
Threshold uncertainty score0.743

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.223
Teacher spread0.217 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations44
Published2010
Admission routes1
Has abstractyes

Explore more

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