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Record W2094116866 · doi:10.1002/macp.200500429

Optical, Electrochemical, Magnetic, and Conductive Properties of New Poly(indolocarbazole‐<i>alt</i>‐bithiophene)s

2006· article· en· W2094116866 on OpenAlex
Nicolas Blouin, Mario Leclerc, Barbara Vercelli, Sandro Zecchin, Gianni Zotti

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueMacromolecular Chemistry and Physics · 2006
Typearticle
Languageen
FieldEngineering
TopicOrganic Electronics and Photovoltaics
Canadian institutionsUniversité Laval
Fundersnot available
KeywordsPolaronCyclic voltammetryBipolaronCopolymerMoietyElectrochemistryPolymer chemistryStille reactionChemistryFluoreneRedoxPhotochemistryConductive polymerQuinoneElectron paramagnetic resonanceMaterials sciencePolymerPhysical chemistryElectrodeInorganic chemistryOrganic chemistryElectronNuclear magnetic resonance

Abstract

fetched live from OpenAlex

Abstract Summary: New alternating copolymers based on indolocarbazole (IC), both two‐ and three‐coupled, and bithiophene (BT) or bis(3,4‐ethylenedioxythiophene) (BiEDOT), were obtained using Stille or Suzuki coupling reactions. Those copolymers have been investigated by cyclic voltammetry, electrochemical quartz crystal microbalance, in situ electron spin resonance, in situ conductivity, and UV‐Vis‐NIR spectroelectrochemistry techniques. All polymer films undergo reversible oxidation processes. One to three isoelectronic oxidation processes, involving one electron per repeat unit, produce radical cations, dications, and radical trications. The oxidative charge is localized in the IC moiety for BT copolymers or over the whole polyconjugated backbone for BiEDOT copolymers. Redox neutral‐polaron conductivities are in the range of 0.02–0.1 S · cm −1 and polaron‐bipolaron conductivities in the range of 0.1–0.7 S · cm −1 . Chemical structure of the PIC derivatives. magnified image Chemical structure of the PIC derivatives.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.014
Threshold uncertainty score0.888

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.164
Teacher spread0.160 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it