Switching of a quantum dot spin valve by single molecule magnets
Bibliographic record
Abstract
We explore theoretically the spin transport in nanostructures consisting of a gold quantum dot bridging nonmagnetic electrodes and two Mn${}_{12}$-Ph single molecule magnets (SMMs) that are thiol bonded to the dot but are not in direct contact with the electrodes. We find that reversal of the magnetic moment of either SMM by the application of a magnetic field leads to a large change in the resistance of the dot, i.e., a strong spin-valve effect. We show that this phenomenon arises from the following physical principle: The spin-dependent molecular orbitals that extend over the dot and both SMMs change drastically when the magnetic moment of either SMM is reversed, resulting in a large change in the conduction via those orbitals. The same physics may also be responsible for the spin-valve phenomena discovered recently in carbon nanotube quantum dots with rare-earth SMMs [M. Urdampilleta et al., Nat. Mater. 10, 502 (2011)].
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How this classification was reachedexpand
Full frame machine prediction
Teacher imitationNot calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.
Distilled classifier scores by category (both heads)
| Category | Codex | Gemma |
|---|---|---|
| Metaresearch | 0.000 | 0.000 |
| Meta-epidemiology (narrow) | 0.000 | 0.000 |
| Meta-epidemiology (broad) | 0.000 | 0.000 |
| Bibliometrics | 0.000 | 0.000 |
| Science and technology studies | 0.000 | 0.001 |
| Scholarly communication | 0.001 | 0.001 |
| Open science | 0.000 | 0.000 |
| Research integrity | 0.001 | 0.000 |
| Insufficient payload (model declined to judge) | 0.002 | 0.000 |
Machine scores (provisional)
The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.
Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.
score_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from itClassification
machine, unvalidatedMachine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.
How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".