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Record W2103902008 · doi:10.1002/hlca.200690277

Investigation of the Interactions of <i>β</i>‐Peptides with DNA Duplexes by Circular Dichroism Spectroscopy

2006· article· en· W2103902008 on OpenAlexaff
Kenji Namoto, James Gardiner, Thierry Kimmerlin, Dieter Seebàch

Bibliographic record

VenueHelvetica Chimica Acta · 2006
Typearticle
Languageen
FieldBiochemistry, Genetics and Molecular Biology
TopicChemical Synthesis and Analysis
Canadian institutionsInstitute of Particle Physics
Fundersnot available
KeywordsChemistryCircular dichroismDNAPeptideSide chainStereochemistryHelix (gastropod)Sequence (biology)Duplex (building)Base pairCrystallographyBiophysicsBiochemistryPolymer

Abstract

fetched live from OpenAlex

Abstract The interaction of β ‐peptides with the DNA duplexes of dA 20 dT 20 and a GCN4‐binding CRE sequence was examined. To gauge the factors that govern these interactions, two β ‐pentadecapeptides, 1 and 2 , a β ‐dodecapeptide, 3 , three β ‐decapeptides, 4 – 6 , three β ‐heptapeptides, 7 – 9 , and β ‐octaarginine 10 were designed and synthesized. The β ‐peptides were conceived to adopt a β ‐peptide 3 14 helix, in which the side chains at position i and i + 3 are aligned vertically along one side of the helix. The side chains of Lys, Asn, and Arg were positioned such that potential H‐bonding sites were created for a helical conformation to interact with the base pairs of DNA. CD Analysis showed that β ‐peptides 1, 2 , and 10 interacted with dA 20 dT 20 . In addition, β ‐peptides 1 and 2 showed significant interaction with a DNA‐duplex 20mer containing the ATF/CREB recognition sequence for the regulatory protein GCN4. It is impossible, at this stage of the investigation, to make a safe proposal about the actual nature of the interaction of the structures(s) of the complexes, the formation of which is suggested by the CD spectra reported herein.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.319

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.198
Teacher spread0.193 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations15
Published2006
Admission routes1
Has abstractyes

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