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Record W2104543407 · doi:10.1109/ceidp.1996.564551

Dynamic decomposition of arced SF/sub 6/ by-products on activated alumina

2002· article· en· W2104543407 on OpenAlexaff
Alain Rochefort, T. Lussier, M. Frechette, R.Y. Larocque

Bibliographic record

Venuenot available
Typearticle
Languageen
FieldMaterials Science
TopicCatalytic Processes in Materials Science
Canadian institutionsHydro-Québec
Fundersnot available
KeywordsAdsorptionDesorptionSaturation (graph theory)Analytical Chemistry (journal)DecompositionChemistryPhase (matter)Materials sciencePhysical chemistryChromatographyOrganic chemistry

Abstract

fetched live from OpenAlex

The dynamic interaction of SOF/sub 2/ with activated alumina has been studied at 298 K in adsorption experiments. The SOF/sub 2/ adsorption process occurs in three distinct regimes related to the available adsorption sites on alumina. The first regime is an adsorption-reaction process where the change observed in the gas phase is essentially a sharp decrease in the amount of SOF/sub 2/. During the SOF/sub 2/ adsorption on alumina, an important fraction of the adsorbed phase is converted into SO/sub 2/. On saturation of the alumina surface with SOF/sub 2/, the amount of desorbing SO/sub 2/ starts to increase in the gas phase as the amount of SOF/sub 2/ decreases. This second regime is characterized by a competitive adsorption-desorption process which involves the adsorption of SOF/sub 2/ simultaneously with the desorption of SO/sub 2/ from a same site. The last regime consists of stabilization in the production of SO/sub 2/ in the gas phase, which could correspond to its equilibrium with the SO/sub 2/-SOF/sub 2/ adsorbed mixture. The typical SOF/sub 2/ adsorption curve is well described by a Langmuir-type adsorption (type I) which gives an adsorption coefficient k/sub a//k/sub d//spl ap/0.4 h/sup -1/.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.254
Teacher spread0.241 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2002
Admission routes1
Has abstractyes

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Same topicCatalytic Processes in Materials ScienceFrench-language works237,207