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Preparation and characterization of N–TiO<sub>2</sub> photocatalyst with high crystallinity and enhanced photocatalytic inactivation of bacteria

2013· article· en· W2107229124 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueNanotechnology · 2013
Typearticle
Languageen
FieldEnergy
TopicTiO2 Photocatalysis and Solar Cells
Canadian institutionsWestern University
Fundersnot available
KeywordsPhotocatalysisAnataseMaterials scienceBrookiteCrystallinityNuclear chemistryVisible spectrumMethylene blueNanoparticleTitaniumChemical engineeringNanotechnologyCatalysisOrganic chemistryChemistryComposite material

Abstract

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This study reports the synthesis, characterization and environmental applications of nitrogen doped TiO2 photocatalyst in the form of powder and film. N-TiO2 photocatalysts were synthesized via the hydrolysis of titanium tetraisopropoxide using urea as the nitrogen source. The crystalline structure, particle size and specific surface area of the resultant N-TiO2 nanoparticles were investigated by x-ray powder diffraction and the Brunauer-Emmett-Teller method. The results showed that a mixture of anatase and brookite phases was formed at pH 1 after annealing the powder at 450 ° C for 4 h, in contrast to a pure anatase phase at pH 3. UV-vis spectral characterization showed that the absorption region of the as-prepared N-TiO2 was extended to the visible light region. Stable sols could be achieved by controlling the molar ratio of water-to-titanium precursor and pH of the sols. During the photocatalytic test, in comparison to the standard commercial photocatalyst Evonik-Degussa P25 and home-made bare TiO2 nanoparticles, the N-TiO2 particles exhibited enhanced photocatalytic performance for degradation of methylene blue (MB) dye. The visible light induced photocatalytic inactivation of the obtained nanopowders and nanofilms on bacteria (Escherichia coli) was evaluated. The N-TiO2 nanomaterials showed higher bactericidal activity under visible light irradiation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.007
Threshold uncertainty score0.696

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.199
Teacher spread0.194 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it